Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 138, Issue 26, Pages 8068-8071Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.6b04206
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Funding
- ERC [258580]
- EPSRC [EP/I004769/1, EP/I004769/2]
- University of Nottingham
- GlaxoSmithKline
- EPSRC [EP/I004769/2, EP/I004769/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/I004769/1, EP/I004769/2, 1498235] Funding Source: researchfish
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Nickel-catalyzed additions of arylboronic acids to alkynes, followed by enantioselective cyclizations of the alkenylnickel species onto tethered ketones or enones, are reported. These reactions are reliant upon the formal anti-carbonickelation of the alkyne, which is postulated to occur by the reversible E/Z isomerization of an alkenylnickel species.
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