Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 138, Issue 18, Pages 5801-5804Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.6b02702
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Funding
- Danish Council for Independent Research [409000201, 12-125226, 10-081659]
- European Commission Initial Training Network MAGIC
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Quantum coherence is detected in the 4f single-ion magnet (SIM) Yb(trensal), by isotope selective pulsed EPR spectroscopy on an oriented single crystal. At X-band, the spin-lattice relaxation (T-1) and phase memory (T-m) times are found to be independent of the nuclei bearing, or not, a nuclear spin. The observation of Rabi oscillations of the spin echo demonstrates the possibility to coherently manipulate the system for more than 70 rotations. This renders Yb(trensal), a sublimable and chemically modifiable SIM, an excellent candidate for quantum information processing.
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