Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 138, Issue 4, Pages 1313-1319Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b11641
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Funding
- EPSRC [EP/K030108/1]
- WPI Initiative of MEXT, Japan
- National University of Defense Technology
- [25620148]
- Engineering and Physical Sciences Research Council [EP/L011972/1, EP/J015067/1, EP/H001972/1, EP/K030108/1, EP/N017188/1] Funding Source: researchfish
- EPSRC [EP/H001972/1, EP/K030108/1, EP/L011972/1, EP/N017188/1, EP/J015067/1] Funding Source: UKRI
- Grants-in-Aid for Scientific Research [14J03432] Funding Source: KAKEN
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Paramagnetic endohedral fullerenes and phthalocyanine (Pc) complexes are promising building blocks for molecular quantum information processing, for which tunable dipolar coupling is required. We have linked these two spin qubit candidates together and characterized the resulting electron paramagnetic resonance properties, including the spin dipolar coupling between the fullerene spin and the copper spin. Having interpreted the distance-dependent coupling strength quantitatively and further discussed the antiferromagnetic aggregation effect of the CuPc moieties, we demonstrate two ways of tuning the dipolar coupling in such dyad systems: changing the spacer group and adjusting the solution concentration.
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