4.8 Review

Emerging Spintronic Materials and Functionalities

Journal

ADVANCED MATERIALS
Volume -, Issue -, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202301854

Keywords

2D materials; chiral-induced spin selectivity; multifunctional spintronic devices; organic-inorganic hybrid perovskites; organic semiconductors

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This article discusses the performance and functionalities of organic semiconductors, organic-inorganic hybrid perovskites, and 2D materials in advanced spintronics applications. The spin transport and spin manipulation properties of these materials are discussed separately, as well as the multifunctionalities arising from photoelectric and chiral-induced spin selectivity. The challenges and future perspectives of using these materials for advanced spintronics development are also presented.
The explosive growth of the information era has put forward urgent requirements for ultrahigh-speed and extremely efficient computations. In direct contrary to charge-based computations, spintronics aims to use spins as information carriers for data storage, transmission, and decoding, to help fully realize electronic device miniaturization and high integration for next-generation computing technologies. Currently, many novel spintronic materials have been developed with unique properties and multifunctionalities, including organic semiconductors (OSCs), organic-inorganic hybrid perovskites (OIHPs), and 2D materials (2DMs). These materials are useful to fulfill the demand for developing diverse and advanced spintronic devices. Herein, these promising materials are systematically reviewed for advanced spintronic applications. Due to the distinct chemical and physical structures of OSCs, OIHPs, and 2DMs, their spintronic properties (spin transport and spin manipulation) are discussed separately. In addition, some multifunctionalities due to photoelectric and chiral-induced spin selectivity (CISS) are overviewed, including the spin-filter effect, spin-photovoltaics, spin-light emitting devices, and spin-transistor functions. Subsequently, challenges and future perspectives of using these multifunctional materials for the development of advanced spintronics are presented. This review aims at discussing the spin-related performance and functionalities of diverse emerging spintronic material systems. The spin transport/manipulation properties of organic semiconductors, organic-inorganic hybrid perovskites, and 2D materials are discussed in the first place, respectively. Following, device multifunctionalities based on these materials are discussed, including spin-filter effect via chiral-induced spin selectivity, spin-photovoltaic, spin-light-emitting, and spin-transistor functions.image

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