A Structure Self-Healing Li-Rich Cathode Achieved by Lithium Supplement of Li-Rich LLZO Coating

Article Nanoscience & Nanotechnology

Surface Engineering and Trace Cobalt Doping Suppress Overall Li/Ni Mixing of Li-rich Mn-based Cathode Materials

Junxin Chen et al.

Summary: Surface modification and Co doping can effectively suppress Li/Ni mixing and improve the electrochemical performance of cathode materials.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

A Redox Couple Strategy Enables Long-Cycling Li- and Mn-Rich Layered Oxide Cathodes by Suppressing Oxygen Release

Qinong Shao et al.

Summary: Introducing an additional redox couple in Li- and Mn-rich layered oxides cathode significantly enhances cycling stability and inhibits oxygen release, with S2- ions playing a crucial role in stabilizing the oxygen lattice. The findings suggest a potential direction to improve the cycling stability of high-energy anion-redox cathode materials for rechargeable metal-ion batteries.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Building Homogenous Li2TiO3 Coating Layer on Primary Particles to Stabilize Li-Rich Mn-Based Cathode Materials

Jiuding Liu et al.

Summary: A facile route to build a Li2TiO3 coating layer on Li-rich Mn-based oxide (LRMO) is reported in this study. The prepared coated LRMO shows improved cycling stability and voltage retention, as well as suppressed oxygen release, phase transition, and interfacial reactions. Furthermore, the coating layer inhibits transition metal dissolution and prevents the crossover effect of transition metals on the lithium anode.

SMALL (2022)

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Review Chemistry, Physical

Insights into Li-Rich Mn-Based Cathode Materials with High Capacity: from Dimension to Lattice to Atom

Shao-Lun Cui et al.

Summary: Research on Li-rich cathode materials shows that understanding the phase transformation process from microscopic to macroscopic levels is crucial for solving capacity decline issues. By focusing on the relationship between dimensions and performance, phase transformation evolution, and anion participation in charge-discharge cycling, high-performance energy storage materials can be designed and structural stability enhanced.

ADVANCED ENERGY MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Countering Voltage Decay, Redox Sluggishness, and Calendering Incompatibility by Near-Zero-Strain Interphase in Lithium-Rich, Manganese-Based Layered Oxide Electrodes

Weitao He et al.

Summary: By constructing a coherent near-zero-strain interphase on the grain boundaries of cathode secondary particles using the reactive infiltration method (RIM), infusing LiAlO2 material, this study demonstrates enhanced electrochemical cyclability, rate capability, and industrial calendaring performance of lithium-rich, manganese-based layered oxides, marking a significant step toward commercial implementation.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Review Chemistry, Physical

Review of modification strategies in emerging inorganic solid-state electrolytes for lithium, sodium, and potassium batteries

Xuyong Feng et al.

Summary: This review article discusses promising inorganic lithium-, sodium-, and potassium-based solid-state electrolytes (SSEs) and strategies to enhance their ionic conductivity, tune interfaces, and prevent dendrites and side reactions. The focus is on understanding the conduction mechanisms, stability, and microstructure of SSEs, as well as developing new synthesis approaches and cell architectures for improved cycling stability.

JOULE (2022)

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Article Nanoscience & Nanotechnology

Li-Deficient Materials-Decoration Restrains Oxygen Evolution Achieving Excellent Cycling Stability of Li-Rich Mn-Based Cathode

Xueqian Ji et al.

Summary: In this study, Li-deficient materials Li0.3NbO2 and (Nb0.62Li0.15)TiO3 were used to improve the electrochemical performance of Li1.2Mn0.54Ni0.13Co0.13O2, including suppressing oxygen evolution, increasing structural stability, and enhancing Li+ diffusion kinetics.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Physical

Restraining the Octahedron Collapse in Lithium and Manganese Rich NCM Cathode toward Suppressing Structure Transformation

Zhou Xu et al.

Summary: This study proposes a facile and efficient surface strategy to stabilize the layered structure of LMRNCM by regulating the chemical bond interaction between the PAN binder and the LMRNCM particles. The experimental results show that this modification strategy can improve the energy density retention, initial Coulombic efficiency, and rate capacity of the LMRNCM samples.

ADVANCED ENERGY MATERIALS (2022)

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Article Nanoscience & Nanotechnology

Mitigation of Oxygen Evolution and Phase Transition of Li-Rich Mn-Based Layered Oxide Cathodes by Coating with Oxygen-Deficient Perovskite Compounds

Yike Lei et al.

Summary: Coating by oxygen-deficient perovskite La0.9Sr0.1CoO3 can effectively improve the cycling performance and voltage stability of Li-rich Mn-based cathode materials, while reducing gas evolution. The coating has a high oxygen vacancy concentration and forms a uniform coating layer.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Understanding the Role of Alumina (Al2O3), Pentalithium Aluminate (Li5AlO4), and Pentasodium Aluminate (Na5AlO4) Coatings on the Li and Mn-Rich NCM Cathode Material 0.33Li2MnO3•0.67Li(Ni0.4Co0.2Mn0.4)O2 for Enhanced Electrochemical Performance

Sandipan Maiti et al.

Summary: The study discusses the active role of alumina, Li-aluminate, and Na-aluminate as surface protection coatings on Li and Mn-rich NCM cathode materials, showing notable improvements in electrochemical behavior. The coated cathodes demonstrate enhanced cycling and rate performances, with Na-aluminate showing exemplary behavior and significantly higher specific capacities compared to uncoated cathodes, as well as lower evolution of gases and transition metals dissolution.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Tunnel Intergrowth LixMnO2 Nanosheet Arrays as 3D Cathode for High-Performance All-Solid-State Thin Film Lithium Microbatteries

Qiuying Xia et al.

Summary: By fabricating tunnel structured LixMnO2 nanosheet arrays as the cathode for thin film lithium batteries at a low temperature, a 3D structure was successfully constructed with high specific capacity, good rate performance, and excellent cycle performance. This outperforms TFBs using cathodes fabricated at high temperature, showing great potential for microelectronic applications.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Full Concentration Gradient-Tailored Li-Rich Layered Oxides for High-Energy Lithium-Ion Batteries

Tianhao Wu et al.

Summary: A new type of lithium-rich layered oxide material was designed in this study, which successfully reduced voltage decay, improved cycle performance, and thermal stability without any material modifications or electrolyte optimizations. The research results demonstrate that the gradient-tailored material can effectively reduce the thermal release of the battery when charged to the maximum voltage.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

Beyond garnets, phosphates and phosphosulfides solid electrolytes: New ceramic perspectives for all solid lithium metal batteries

Daniele Campanella et al.

Summary: Solid-state electrolytes, as a promising solution for lithium batteries, have advantages over traditional organic electrolytes in terms of Li-metal electrodes affinity and global battery safety, but still face limitations such as moisture sensitivity and partial incompatibility with active materials. Hence, researchers are exploring alternative chemistries and configurations to overcome these deficiencies.

JOURNAL OF POWER SOURCES (2021)

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Article Green & Sustainable Science & Technology

LiMnO2 cathode stabilized by interfacial orbital ordering for sustainable lithium-ion batteries

Xiaohui Zhu et al.

Summary: Global deployments of lithium-ion batteries are set to increase significantly in the future, with a focus on sustainability and replacing cobalt with abundant and environmentally friendly elements such as manganese. The study presents a new strategy for utilizing abundant elements like manganese in battery chemistry for enhanced sustainability, specifically focusing on LiMnO2 cathodes with engineered Mn 3d orbitals orientation.

NATURE SUSTAINABILITY (2021)

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Article Chemistry, Physical

Na-substitution induced oxygen vacancy achieving high transition metal capacity in commercial Li-rich cathode

Quanxin Ma et al.

Summary: This study proposes a method of creating surface oxygen vacancies and Na doping to enhance the structural stability of Li-rich layered Mn-based oxides (LLMOs), leading to improved electrochemical performance. The optimized Na0.1LLMO cathode material shows high initial coulombic efficiency and excellent cycling stability, voltage retention, and rate performance. Pouch cell investigation further confirms the practical applicability of Na-doped LLMO cathode materials on a larger scale.

NANO ENERGY (2021)

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Review Chemistry, Multidisciplinary

Challenges and Recent Advances in High Capacity Li-Rich Cathode Materials for High Energy Density Lithium-Ion Batteries

Wei He et al.

Summary: Li-rich cathode materials have high reversible discharge capacity, but face issues like low kinetic properties and inefficient voltage fading. Advanced technologies and innovative strategies are being developed to address these challenges and improve the performance of these materials for practical applications.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

Lithium-rich manganese-based cathode materials with highly stable lattice and surface enabled by perovskite-type phase-compatible layer

Han-xin Wei et al.

Summary: By modifying the surface of Li-rich Mn-based cathode materials with a perovskite-type LaMnO3 layer, the anion activity was effectively suppressed and cycle stability was improved, leading to enhanced electrochemical performance.

NANO ENERGY (2021)

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Article Chemistry, Physical

Optimized activation of Li2MnO3 effectively boosting rate capability of xLi2MnO3•(1-x)LiMO2 cathode

Youchen Hao et al.

Summary: Introducing trace Bi-doping can improve the voltage decaying issue and enhance cyclability of Li-rich Mn-based oxide cathodes. However, the poor rate capability of LMO is still influenced by the Li2MnO3 phase, restricting its performance.

NANO ENERGY (2021)

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Article Materials Science, Multidisciplinary

Recent breakthroughs and perspectives of high-energy layered oxide cathode materials for lithium ion batteries

Junxiang Liu et al.

Summary: Ni-rich layered oxides (NRLOs) and Li-rich layered oxides (LRLOs) are promising cathode materials for lithium ion batteries (LIBs) due to their high energy density, low cost, and environmental friendliness. However, they face similar challenges such as capacity fading and different obstacles like thermal runaway for NRLOs and voltage decay for LRLOs. Strategies to improve their performance from different scales including ion-doping, microstructure designs, particle modifications, and electrode/electrolyte interface engineering are essential for their development.

MATERIALS TODAY (2021)

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Article Chemistry, Multidisciplinary

Phase Compatible NiFe2O4 Coating Tunes Oxygen Redox in Li-Rich Layered Oxide

Jiming Peng et al.

Summary: A surface-coating strategy using NiFe2O4 was developed to enhance the performance of Li-rich layered oxides in lithium-ion batteries, resulting in improved cycle stability and rate capability. This strategy effectively traps surface lattice oxygen and restrains cation migration, decoupling the surface oxygen redox from cation movement.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

A Universal Strategy toward the Precise Regulation of Initial Coulombic Efficiency of Li-Rich Mn-Based Cathode Materials

Weibin Guo et al.

Summary: This study proposes a simple interface engineering method to effectively improve the initial Coulombic efficiency and rate performance of LRM. By introducing cation/anion double defects and in situ surface reconstruction layer, the diffusion barrier of Li+ ions can be reduced and the surface lattice oxygen can be stabilized. This simple interface engineering method is universal and can effectively enhance the ICE of other types of LRM.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

Achieving high initial coulombic efficiency and low voltage dropping in Li-rich Mn-based cathode materials by Metal-Organic frameworks-derived coating

Chao Huang et al.

Summary: The study presents a facile Metal-Organic Frameworks self-assembly coating strategy to modify Li-rich Mn-based oxides, improving their performance and enhancing the capacity retention of the batteries.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Physical

Inhibiting Oxygen Release from Li-rich, Mn-rich Layered Oxides at the Surface with a Solution Processable Oxygen Scavenger Polymer

Se Young Kim et al.

Summary: The performance of Li-rich Mn-rich layered cathode material is enhanced by scavenging evolved oxygen species with a polydopamine surface coating, resulting in improved rate capability and diminished capacity fading during cycling.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Applied

Suppress voltage decay of lithium-rich materials by coating layers with different crystalline states

Zhiwei Zhou et al.

Summary: The use of different crystalline states of ZrO2 as coating layers improves the electrochemical performance of Li[Li0.2Mn0.54Ni0.13Co0.13]O-2 materials. The polycrystal ZrO2 coating layer shows an advantage in rate performance, while the single crystal ZrO2-coating layer exhibits better cycling performance.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Review Chemistry, Physical

Interphase Engineering by Electrolyte Additives for Lithium-Rich Layered Oxides: Advances and Perspectives

Jingteng Zhao et al.

Summary: This review paper summarizes the research progress in functional electrolyte additives for LLOs, discusses the mechanisms of CEI construction, and tentatively proposes suggestions to promote the large-scale application of LLOs for LIBs through screening and customizing electrolyte additives.

ACS ENERGY LETTERS (2021)

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Article Chemistry, Physical

Modified Li7La3Zr2O12 (LLZO) and LLZO-polymer composites for solid-state lithium batteries

Wanzheng Lu et al.

Summary: SSLB is regarded as a promising candidate for energy storage devices, with LLZO solid-state electrolyte playing a key role, and significant progress has been made in research, although challenges remain to be addressed.

ENERGY STORAGE MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Boosting the Electrochemical Performance of Li- and Mn-Rich Cathodes by a Three-in-One Strategy

Wei He et al.

Summary: This study proposes a three-in-one method combining cation-polyanion co-doping, defect construction, and stress engineering to address the capacity loss, structural mismatch, and stress accumulation issues in Li- and Mn-rich cathodes. The co-doped Na+/SO42- stabilizes the framework, enhances capacity and voltage stability, while induced defects activate more reaction sites and improve electrochemical performance. The unique defect bands and crystal bands structure alleviate stress accumulation, resulting in high-capacity retention and low voltage attenuation after cycling.

NANO-MICRO LETTERS (2021)

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Article Chemistry, Multidisciplinary

Foldable potassium-ion batteries enabled by free-standing and flexible SnS2@C nanofibers

Deping Li et al.

Summary: The study confines SnS2 in N, S co-doped carbon nanofibers as anode materials for potassium-ion batteries, demonstrating high performance and stability. Through experiments and theoretical calculations, the synergistic effects of the N, S co-doping strategy in boosting K-ion transport kinetics are revealed.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review Chemistry, Physical

Solid-State Li-Metal Batteries: Challenges and Horizons of Oxide and Sulfide Solid Electrolytes and Their Interfaces

Kun Joong Kim et al.

Summary: The introduction of new, safe, and reliable solid-electrolyte chemistries and technologies can potentially overcome the challenges facing their liquid counterparts while widening the breadth of possible applications. Through analyzing the transition from liquid-based Li-ion batteries (LIBs) to all-solid-state Li-metal batteries (ASSLBs), a roadmap for the development of a successful oxide and sulfide-based ASSLB is introduced, focusing on interfacial challenges and considering parameters such as energy density, power density, longterm stability, processing, and safety.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Voltage decay and redox asymmetry mitigation by reversible cation migration in lithium-rich layered oxide electrodes

Donggun Eum et al.

NATURE MATERIALS (2020)

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Structural evolution at the oxidative and reductive limits in the first electrochemical cycle of Li1.2Ni0.13Mn0.54Co0.13O2

Ei Yin et al.

NATURE COMMUNICATIONS (2020)

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Article Chemistry, Multidisciplinary

Local Electric-Field-Driven Fast Li Diffusion Kinetics at the Piezoelectric LiTaO3 Modified Li-Rich Cathode-Electrolyte Interphase

Mengting Si et al.

ADVANCED SCIENCE (2020)

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Editorial Material Multidisciplinary Sciences

A retrospective on lithium-ion batteries

Jing Xie et al.

NATURE COMMUNICATIONS (2020)

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Activation and stabilization mechanisms of anionic redox for Li storage applications: Joint experimental and theoretical study on Li2TiO3-LiMnO2 binary system

Yuki Kobayashi et al.

MATERIALS TODAY (2020)

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Pseudo-Bonding and Electric-Field Harmony for Li-Rich Mn-Based Oxide Cathode

Jun Chen et al.

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Structural Distortion Induced by Manganese Activation in a Lithium-Rich Layered Cathode

Liguang Wang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Lithium-rich layered oxide nanowires bearing porous structures and spinel domains as cathode materials for lithium-ion batteries

Boda Deng et al.

JOURNAL OF POWER SOURCES (2019)

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Dual conductive surface engineering of Li-Rich oxides cathode for superior high-energy-density Li-Ion batteries

Fu-Da Yu et al.

NANO ENERGY (2019)

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Surface-to-Bulk Redox Coupling through Thermally Driven Li Redistribution in Li- and Mn-Rich Layered Cathode Materials

Shaofeng Li et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Surface-Functionalized Coating for Lithium-Rich Cathode Material To Achieve Ultra-High Rate and Excellent Cycle Performance

Yanying Liu et al.

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Tuning Oxygen Redox Chemistry in Li-Rich Mn-Based Layered Oxide Cathodes by Modulating Cation Arrangement

Jicheng Zhang et al.

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Improving electrochemical performance of lithium-rich cathode material Li1.2Mn0.52Ni0.13Co0.13W0.02O2 coated with Li2WO4 for lithium ion batteries

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Lithium-Metal Growth Kinetics on LLZO Garnet-Type Solid Electrolytes

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A Structure Self-Healing Li-Rich Cathode Achieved by Lithium Supplement of Li-Rich LLZO Coating

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