Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 138, Issue 32, Pages 10120-10123Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.6b06546
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Funding
- National Science Foundation
- Georgia Tech Facilitating Academic Careers in Engineering and Science (GT-FACES)
- American Chemical Society [55562-DNI7]
- Ohio State University
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Finding new ways to construct crystalline multiple-component covalent organic frameworks (COFs) has become an important focus. Herein we report the synthesis of three novel COFs containing a homogeneous and heterogeneous distribution of pi-conjugated dehydrobenzoannulene (DBA) vertex units. The COFs were synthesized by reacting different tatios of C-3-syrninetric DBA catechol, monomers with C-2-symmetric pyrene-2,7dibotonic acid (PDBA) to yield three COFs, Py-DBACOF 1, Py-DBA-COF 2, and Py-MV-DBA-COF. All three materials are highly crystalline and display unique luminescent properties in the solid state.
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