4.7 Article

Thermoplastic and Electrically Conductive Fibers for Highly Stretchable and Sensitive Strain Sensors

Journal

ACS APPLIED POLYMER MATERIALS
Volume 4, Issue 12, Pages 8795-8802

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsapm.2c01199

Keywords

liquid metal; polyurethane; fiber; gauge factor; wearable electronics

Funding

  1. National Natural Science Foundation of China
  2. [52173249]

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This work presents the fabrication of a highly sensitive and stretchable fiber sensor, STF, using thermoplastic polyurethane integrated with semi-liquid metal. The study also discovers the adhesive properties of thermoplastic polyurethane, allowing for the construction of diverse fiber structures that enhance the sensor's performance. The rapid response capability of STF makes it suitable for monitoring human motion.
Stretchable and conductive fibers have attracted immense interest in the fields of electronic skin, smart textiles, and environmental monitoring due to their inherited unique characteristics. Although various types of stretchable fibers have been investigated, the complicated fabrication and high cost of the specifically designed fibers have greatly hindered the broad applications of the sensors. This work reports the use of thermoplastic polyurethane (TPU) integrated with a semiliquid metal (SLM) to fabricate SLM-TPU fiber (namely, STF) through traditional melt extrusion. The interaction between SLM and TPU enables STF to be highly sensitive (gauge factor (GF): 177-240) and stretchable (strain: 421%) resistive sensor. Besides, this work discovers that TPU could act as an effective adhesive to conveniently construct different structures from the fibers, such as hexagonal-prism, double-helix and mesh textures. These diverse structures enhance the tensile strength and strain of STF. In addition, the phenomenal sensitivity and stretchability make the STF a rapid-response strain sensor with the ability to monitor human motion.

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