4.6 Article

CsPbBr3 Perovskite Nanocrystals for a Q-Switched Pulsed Fiber Laser in the C-Band Region

Journal

ACS OMEGA
Volume -, Issue -, Pages -

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsomega.2c06107

Keywords

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Funding

  1. Natural Science Foundation of Inner Mongolia of China
  2. Research Foundation for Advanced Talents of Inner Mongolia Normal University
  3. Research Project of the Inner Mongolia University of Technology
  4. Scientific Research Startup Fund of Inner Mongolia University of Technology
  5. Natural Science Foundation of Jilin Province
  6. [2021BS02019]
  7. [2020YJRC012]
  8. [ZZ202108]
  9. [DC2200000916]
  10. [YDZJ202201ZYTS324]

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In this study, passively Q-switched erbium-doped fiber laser (EDFL) operation at the C-band region was achieved using perovskite CsPbBr3 nanocrystals as a saturable absorber (SA). The CsPbBr3 nanocrystals exhibited broadband linear optical absorption in the 300-2000 nm range and nonlinear optical absorption at the C-band range of around 1560 nm.
All-inorganic perovskite nanocrystals have been widely reported as promising light-harvesting and light-emitting semiconductor nanomaterials. However, their nonlinear optical properties and laser applications have rarely been explored, especially for pulse laser modulation in the telecommunication C-band window. Herein, we experimentally demonstrated a passively Q-switched erbium-doped fiber laser (EDFL) operation at the C-band region using perovskite CsPbBr3 nanocrystals as a saturable absorber (SA). The broadband linear optical absorption in the 300-2000 nm range and the nonlinear optical absorption at the C-band range of around 1560 nm were discovered and investigated in CsPbBr3 nanocrystals. The CsPbBr3-based SA exhibited good saturable absorption performance with a modulation depth and saturation intensity equivalent to 19.1% and 10.9 MW/cm2, respectively. By integrating the CsPbBr3 SA into an EDFL cavity, a passively Q-switched operation with a central wavelength of 1560 nm, a threshold pump power of 60 mW, and the shortest pulse duration of 5.96 mu s was achieved. In addition, such a Q-switching operation exhibited long-term stability. Our results indicate that the CsPbBr3 perovskite nanocrystals can serve as an efficient candidate for constructing pulsed lasers in the C-band or even longer NIR wavelength region.

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