4.8 Article

Carrier-Density Control of the SrTiO3 (001) Surface 2D Electron Gas studied by ARPES

Journal

ADVANCED MATERIALS
Volume 27, Issue 26, Pages 3894-+

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201501556

Keywords

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Funding

  1. Swiss National Science Foundation [200021-146995]
  2. UK-EPSRC [EP/I031014/1]
  3. Royal Society
  4. Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan [24224009]
  5. Swiss National Science Foundation (SNF) [200021_146995] Funding Source: Swiss National Science Foundation (SNF)
  6. EPSRC [EP/I031014/1] Funding Source: UKRI
  7. Engineering and Physical Sciences Research Council [EP/I031014/1] Funding Source: researchfish

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The origin of the 2D electron gas (2DEG) stabilized at the bare surface of SrTiO3 (001) is investigated. Using high-resolution angle-resolved photoemission and core-level spectroscopy, it is shown conclusively that this 2DEG arises from light-induced oxygen vacancies. The dominant mechanism driving vacancy formation is identified, allowing unprecedented control over the 2DEG carrier density.

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