Journal
ACS SENSORS
Volume 8, Issue 1, Pages 122-132Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acssensors.2c01845
Keywords
2D materials; gas sensors; graphene; hBN; heterostructures
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The development of graphene-hBN heterostructures in electronic and gas sensing devices has sparked research interest. Eddy current measurements show lower sheet conductance in graphene-hBN heterostructures compared to previously reported results obtained through contact-based methods. Chemiresistive measurements reveal different incremental sheet conductance responses and sign variations in graphene and graphene-hBN sensors during oxygen adsorption, highlighting the importance of hysteresis in sensing processes.
The development of graphene-based electronic and gas sensing devices has motivated considerable research interest in the properties of graphene-hBN heterostructures. Eddy current measurements of the sheet conductance of graphene-hBN heterostructures show a relatively low conductance, as compared to results previously reported in the literature, all of which were obtained using contact-based measurement methods. Chemiresis-tive measurements of the graphene-hBN heterostructure response to oxygen adsorption, including hysteric effects under transient multicycle loading, show that the incremental sheet conductance responses of graphene and graphene-hBN sensors differ in sign. A transient, nonlinear, history dependent constitutive model of graphene-hBN response to oxygen adsorption distinguishes stochastic variations in material properties from deterministic variations in sensor performance. The deterministic variations are due to sensing process hysteresis, a phenomenon of central interest in the development of graphene-based sensor systems.
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