Journal
PHYSICAL REVIEW APPLIED
Volume 19, Issue 1, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevApplied.19.L011001
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In this study, nitrogen-doped porous graphene metamaterials on the nanoscale are designed using a topological kirigami assembly, with a thermal-switching ratio of 27.79, which is more than double the value of previous work. The excellent performance is attributed to the chiral folding-unfolding deformation, resulting in a metal-insulator transition. This research provides a nanomaterial design paradigm that bridges the gap between kinematics and functional metamaterials, motivating the development of high-performance thermal regulators.
One of the current challenges in nanoscience is tailoring phononic devices, such as thermal regu-lators and thermal computing. This has long been a rather elusive task because the thermal-switching ratio is not as high as electronic analogs. Mapping from a topological kirigami assembly, nitrogen-doped porous graphene metamaterials on the nanoscale are inversely designed with a thermal-switching ratio of 27.79, which is more than double the value of previous work. We trace this behavior to the chiral folding-unfolding deformation, resulting in a metal-insulator transition. This study provides a nanomate-rial design paradigm to bridge the gap between kinematics and functional metamaterials that motivates the development of high-performance thermal regulators.
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