4.7 Article

Improved Electrical Properties of EHD Jet-Patterned MoS2 Thin-Film Transistors with Printed Ag Electrodes on a High-k Dielectric

Journal

NANOMATERIALS
Volume 13, Issue 1, Pages -

Publisher

MDPI
DOI: 10.3390/nano13010194

Keywords

MoS2; Ag electrode; EHD jet printing; high-k dielectric; thin-film transistors

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EHD jet printing is a versatile method to print materials with a wide viscosity range. In this work, solution-based MoS2 and high-viscosity Ag paste were successfully printed using EHD jet printing for electronic applications. MoS2 TFTs with patterned Ag source and drain were fabricated using low-k silica and high-k alumina gate dielectrics. Devices based on Al2O3 exhibited much better electrical properties than those based on SiO2, with an improvement of around one order of magnitude in hysteresis after changing the gate insulator material.
Electrohydrodynamic (EHD) jet printing is known as a versatile method to print a wide viscosity range of materials that are impossible to print by conventional inkjet printing. Hence, with the understanding of the benefits of EHD jet printing, solution-based MoS2 and a high-viscosity Ag paste were EHD jet-printed for electronic applications in this work. In particular, printed MoS2 TFTs with a patterned Ag source and drain were successfully fabricated with low-k silica (SiO2) and high-k alumina (Al2O3) gate dielectrics, respectively. Eventually, the devices based on Al2O3 exhibited much better electrical properties compared to the ones based on SiO2. Interestingly, an improvement of around one order of magnitude in hysteresis was achieved for devices after changing the gate insulator from SiO2 to Al2O3. In effect, the results of this work for the printed MoS2 and the printed Ag source and drains for TFTs demonstrate a new approach for jet printing in the fabrication of electronic devices.

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