4.8 Article

Gradient-Induced Dzyaloshinskii-Moriya Interaction

Journal

NANO LETTERS
Volume 22, Issue 24, Pages 10128-10133

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.2c03973

Keywords

composition gradient; DMI; skyrmion; field-free SOT switching

Funding

  1. National Key Research and Development Program of China (MOST) [2022YFA1405102]
  2. National Natural Science Foundation of China [11874059, 12174405]
  3. Key Research Program of Frontier Sciences, CAS [ZDBS-LY-7021]
  4. Ningbo Key Scientific and Technological Project [2021000215]
  5. Pioneer and Leading Goose R&D Program of Zhejiang Province [2022C01053]
  6. Zhejiang Provincial Natural Science Foundation [LR19A040002]
  7. Beijing National Laboratory for Condensed Matter Physics [2021000123]
  8. Ningbo Natural Science Foundation [2021J226]
  9. European Union [881603]

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In this study, we used atomistic spin calculations to investigate an intriguing type of Dzyaloshinskii-Moriya interaction (DMI) that emerges in films with composition gradient. We found that the strength and chirality of this DMI can be controlled by the composition gradient, even in disordered systems. Our study also demonstrated the DMI-induced chiral magnetic structures and field-free spin-orbit torque switching, both of which are crucial for practical device applications.
The Dzyaloshinskii-Moriya interaction (DMI) that arises in the magnetic systems with broken inversion symmetry plays an essential role in topological spintronics. Here, by means of atomistic spin calculations, we study an intriguing type of DMI (g-DMI) that emerges in the films with composition gradient. We show that both the strength and chirality of g-DMI can be controlled by the composition gradient even in the disordered system. The layerresolved analysis of g-DMI unveils its additive nature inside the bulk layers and clarifies the linear thickness dependence of g-DMI observed in experiments. Furthermore, we demonstrate the g-DMI-induced chiral magnetic structures, such as spin spirals and skyrmions, and the g-DMI driven field-free spin-orbit torque (SOT) switching, both of which are crucial toward practical device application. These results elucidate the underlying mechanisms of g-DMI and open up a new way to engineer the topological magnetic textures.

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