Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 87, Issue 24, Pages 16928-16936Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.2c02312
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Funding
- National Science Foundation under MRI Grant [CHE-2117256]
- National Science Foundation [DMR-1752782]
- University of Tampa through the Department of Chemistry, Biochemistry Physics (UT)
- University of Tampa through Research Innovation and Scholarly Excellence Grant (UT)
- University of Tampa through Undergraduate Research and Inquiry Grant (UT)
- University of Tampa through Summer Undergraduate Research Fellowship
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The electron-donating capabilities of carbazoles have sparked interest in their use as photoinduced single-electron reductants. By manipulating the structure, a better understanding of their reactivity and broader application scope can be achieved. In this study, eight carbazole derivatives were synthesized, characterized, and evaluated as single-electron photoreductants in the hydrodehalogenation of aryl halides and arylation of N-methylpyrrole.
The electron-donating capabilities of carbazoles have stimulated interest in their use as photoinduced single-electron reductants. Due to the modularity of the carbazole, a further broadening and understanding of their reactivity could be achieved by manipulating the structure. Herein, eight carbazole derivatives were synthesized, characterized, and assessed as single-electron photoreductants in the hydrodehalogenation of aryl halides and the arylation of N-methylpyrrole.
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