Adsorptive and photocatalytic performance of cobalt-doped ZnTiO3/Ti3C2Tx MXene nanohybrids towards tetracycline: Kinetics and mechanistic insight

Article Engineering, Environmental

Photocatalytic degradation of tetracycline antibiotic by a novel Bi2Sn2O7/Bi2MoO6 S-scheme heterojunction: Performance, mechanism insight and toxicity assessment

Shijie Li et al.

Summary: Novel Bi2Sn2O7/Bi2MoO6 step-scheme heterojunctions were fabricated, which could effectively degrade tetracycline antibiotics and showed no toxicity.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Environmental Sciences

Enhanced photocatalytic activity of two dimensional ternary nanocomposites of ZnO-Bi2WO6-Ti3C2 MXene under natural sunlight irradiation

Vishal Sharma et al.

Summary: The study presents a novel 2D ternary photocatalyst ZnO-Bi2WO6-Ti3C2 prepared through a two-step electrostatic assembly route, which demonstrated high efficiency in degrading the colorless pharmaceutical pollutant ciprofloxacin under natural sunlight irradiation, with a maximum degradation rate of around 77% in 160 minutes. Mechanistic investigation revealed the significant role of MXene in separating photogenerated charges within the photocatalyst.

CHEMOSPHERE (2022)

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Article Engineering, Environmental

Strong adsorption properties and mechanism of action with regard to tetracycline adsorption of double-network polyvinyl alcohol-copper alginate gel beads

Quan Liao et al.

Summary: Glutaraldehyde was used as a hydrophobic modifier to crosslink polyvinyl alcohol (PVA), while copper ions were immobilized by sodium alginate (SA) in this study. The resulting PVA-CA gel beads demonstrated high adsorption capacity for tetracycline (TC) in aqueous solutions, with a maximum adsorption capacity of 231.431 mg/g under optimal conditions. The adsorption process followed pseudo-second-order kinetic and Langmuir isothermal models, and was found to be spontaneous and endothermic. Additionally, cation bonding bridge reactions were identified as the main driving force behind the adsorption mechanism.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Engineering, Environmental

Efficient photocatalytic degradation of sulfasalazine and reduction of hexavalent chromium over robust In2S3/Nd2O3 heterojunction under visible light

M. Murugalakshmi et al.

Summary: In this study, a novel visible light driven heterojunction photocatalyst of In2S3/xNd(2)O(3) nano-composites was designed and synthesized via a simple two-step process. The prepared materials exhibited efficient photocatalytic activity for the double role photooxidation of sulfasalazine and photoreduction of Cr(VI) under visible light illumination. The enhanced efficiency was attributed to the proper band alignment and intimate interfacial contact in the In2S3/10 wt% Nd2O3 p-n heterojunction, which facilitated better charge separation and transfer. The photocatalyst also showed superior photostability and recyclability.

JOURNAL OF WATER PROCESS ENGINEERING (2022)

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Article Engineering, Environmental

Remarkable adsorption for hazardous organic and inorganic contaminants by multifunctional amorphous core-shell structures of metal-organic framework-alginate composites

Lewis Kamande Njaramba et al.

Summary: Novel metal-organic framework-alginate composite beads (CA-MIL-53-AC) were synthesized and used for selective removal of DDT, As(V), and fluoride from water. The composite beads showed excellent adsorption performance and could be regenerated for repeated use. The adsorption process followed pseudo-first-order kinetics and Langmuir/Freundlich isotherms. The adsorption mechanisms involved hydrophobic and pi-pi interactions, ion exchange, surface complexation, and hydrogen bonding.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Environmental Sciences

One-step fabrication of novel MIL-53(Fe, Al) for synergistic adsorption-photocatalytic degradation of tetracycline

Xueqi Chen et al.

Summary: Bimetallic MOFs (MIL-53 (Fe, Al)) were fabricated via a one-step solvothermal method and showed excellent performance in the removal of tetracycline from aqueous solutions. The optimum molar ratio of the bimetallic synthetic was found to be 3:2 (40%MIL-53(Fe, Al)). The 40%MIL-53(Fe, Al) catalyst exhibited high adsorption capacity and photocatalytic synergy, and maintained good stability after multiple cycles.

CHEMOSPHERE (2022)

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Article Engineering, Multidisciplinary

2D/2D nitrogen-rich graphitic carbon nitride coupled Bi2WO6 S-scheme heterojunction for boosting photodegradation of tetracycline: Influencing factors, intermediates, and insights into the mechanism

Karunamoorthy Saravanakumar et al.

Summary: A novel two-dimensional 2D/2D Bi2WO6@g-C3N5 (BiW@CN) heterojunction with remarkable light-harvesting capability and enhanced photocatalytic performance for tetracycline degradation was designed and fabricated. The excellent enhancement activity of BiW@CN is attributed to the formation of an S-scheme heterojunction, promoting spatial charge separation and endowing reduction power to photogenerated electrons. This research provides a new platform for efficient 2D/2D S-scheme heterojunctions for environmental water pollution treatments.

COMPOSITES PART B-ENGINEERING (2022)

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Article Engineering, Chemical

Surface Complexation Enhanced Adsorption of Tetracycline by ALK-MXene

Xuan Dao et al.

Summary: The removal of tetracycline antibiotics from wastewater is an important environmental issue, and this study focused on the use of ALK-MXene with a hydroxyl-rich surface to effectively remove tetracycline. The presence of metal ions was found to enhance the adsorption capacity of tetracycline, with Ni(II) leading to a 750% increase in removal capacity. The adsorption mechanism followed the Freundlich model, and surface modification of metal ions played a key role in enhancing surface complexation.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2022)

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Review Engineering, Environmental

Critical review on adsorptive removal of antibiotics: Present situation, challenges and future perspective

Divyanshi Mangla et al.

Summary: This review provides a thorough understanding of contamination levels, sources, and biological hazards associated with various classes of antibiotics in consumable water. It emphasizes the use of unconventional adsorbents to replace traditional ones with higher efficiency in antibiotic removal.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Engineering, Environmental

Effect of single and multilayered Ti3C2TX MXene as a catalyst and adsorbent on enhanced sonodegradation of diclofenac and verapamil

Sewoon Kim et al.

Summary: In this study, single-layer and multilayer Ti3C2TX MXene were used as catalysts in the ultrasonic treatment, showing increased production of free OH· and enhanced performance due to adsorption. The ultrasonic treatment in the presence of multilayer MXene exhibited the highest synergy effect, by improving dispersion and reducing size.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Engineering, Environmental

Visible-light driven sonophotocatalytic removal of tetracycline using Ca-doped ZnO nanoparticles

Alejandro Bembibre et al.

Summary: The study explores the efficient mineralization of tetracycline antibiotics using Ca-doped ZnO nanopowders under LED visible light and ultrasound irradiation. The catalyst exhibited high efficiency, reusability, and minimal sonophotocorrosion, especially in natural waters' pH range.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Materials Science, Ceramics

Two-dimensional (2D) Ti3C2Tx MXene nanosheets with superior adsorption behavior for phosphate and nitrate ions from the aqueous environment

Perumal Karthikeyan et al.

Summary: The study demonstrated that 2D MXene materials can effectively remove phosphate and nitrate ions from water through various interactions mechanisms. Experimental results indicated that MXenes could be promising adsorbents for toxic ion removal from water/wastewater.

CERAMICS INTERNATIONAL (2021)

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Article Engineering, Environmental

One-step synthesis of nitrogen and sulfur co-doped mesoporous graphite-like carbon nanosheets as a bifunctional material for tetracycline removal via adsorption and catalytic degradation processes: Performance and mechanism

Ke Zhu et al.

Summary: In this study, nitrogen and sulfur co-doped mesoporous graphite-like carbon nanosheets were synthesized and exhibited outstanding removal capacity for tetracycline. The introduction of sulfur significantly adjusted the electron density of the carbon lattice, promoting both tetracycline adsorption and persulfate activation.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Highly efficient photocatalytic degradation of different hazardous contaminants by CaIn2S4-Ti3C2Tx Schottky heterojunction: An experimental and mechanism study

Zhihao Zhuge et al.

Summary: The study synthesized CaIn2S4/MXene Ti3C2Tx Schottky heterojunctions and applied them for photocatalytic degradation and reduction reactions of hazardous contaminants. Ti3C2Tx as a cocatalyst improved the photocatalytic efficiency and the Ti3C2Tx-CaIn2S4 hybrids exhibited outstanding photostability under experimental conditions, showing potential for practical use.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Rational design of a novel LaFeO3/g-C3N4/BiFeO3 double Z-scheme structure: Photocatalytic performance for antibiotic degradation and mechanistic insight

Karunamoorthy Saravanakumar et al.

Summary: A novel ternary symmetric double Z-scheme LaFeO3/g-C3N4/BiFeO3 (LCB) heterojunction nanocomposite was synthesized using a wet chemical process, showing outstanding photocatalytic performance for ciprofloxacin degradation. The enhanced performance is attributed to improved light absorption capability, effective spatial separation, and prolonged charge carriers lifetime in the double Z-scheme system.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Environmental Sciences

Occurrence, fate, and risk assessment of typical tetracycline antibiotics in the aquatic environment: A review

Longyao Xu et al.

Summary: Tetracyclines, widely used as antibiotics, are excreted in large quantities into the environment, causing adverse effects on both ecological systems and human health. This article summarizes the environmental occurrence and behaviors of tetracyclines in aquatic environments, as well as their toxicities and potential risks.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Chemistry, Physical

Hierarchical CoTiO3 microrods on Ti3C2Tx MXene heterostructure as an efficient sonocatalyst for bisphenol A degradation

Karunamoorthy Saravanakumar et al.

Summary: CoTiO3 microrods decorated on MXene nanosheets (CoT@MX) were synthesized via liquid self-assembly method for BPA degradation, displaying superior sonocatalytic activity with a removal efficiency of 96.9%. MXene nanosheets provided new surface-active sites facilitating the interaction between catalyst and BPA pollutant molecules, with (OH)· and O2· contributing to BPA degradation. The feasible sonocatalytic reaction mechanism of CoT@MX was elucidated.

JOURNAL OF MOLECULAR LIQUIDS (2021)

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Article Engineering, Environmental

Enhanced adsorption performance for selected pharmaceutical compounds by sonicated Ti3C2TX MXene

Sewoon Kim et al.

Summary: This study evaluated the adsorption performance of MXene for pharmaceutical compounds, showing the best adsorption of AMT at pH 7. Sonication significantly enhanced the adsorption performance of MXene, with lower frequencies demonstrating better effects.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Catalytic oxidation of naproxen in cobalt spinel ferrite decorated Ti3C2Tx MXene activated persulfate system: Mechanisms and pathways

Aqsa Fayyaz et al.

Summary: Naproxen (NPX) is a nonsteroidal anti-inflammatory drug that can have detrimental effects on human and ecosystem health at certain concentrations in aqueous environments. A nanocatalyst composed of MXene nanosheets and CoFe2O4 nanoparticles was successfully fabricated for the degradation of NPX, with high removal efficiency achieved. Radical and nonradical pathways were found to be involved in the catalytic degradation process, indicating the promising potential of CoFe2O4@MXene/PS system for treating water polluted with NPX.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Environmental Sciences

Strategic combination of ultra violet-visible-near infrared light active materials towards maximum utilization of full solar spectrum for photocatalytic chromium reduction

Abhishek Jain et al.

Summary: Maximizing the utilization of the full solar spectrum in photocatalysis is essential for renewable energy sources and environmental health. A strategic combination of materials has been successfully utilized for chromium reduction, paving the way for the design of more efficient photocatalytic systems.

CHEMOSPHERE (2021)

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Article Chemistry, Physical

Construction of hexagonal nickel-cobalt oxide nanosheets on metal-organic frameworks based on MXene interlayer ion effect for hybrid supercapacitors

Jiaheng Wang et al.

Summary: Designing and adjusting materials with reasonable microscopic morphology is crucial for improving electrochemical performance and assembling hybrid supercapacitors. In this study, nanosheets with a unique hexagonal morphology were prepared, showing excellent capacity retention rate and specific capacity.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Chemistry, Physical

Comparison of the photocatalytic activity of perovskite structures: Bismuth, barium, and zinc titanate nanostructures for photodegradation of methylene blue from water

Gholamreza Pirgholi-Givi et al.

Summary: This study aimed to enhance the photocatalytic performance of TiO2 in the visible light range using TiO2-based nanostructures. The bismuth titanate nanostructures exhibited higher photocatalytic activity among the prepared samples in the visible light range.

JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY (2021)

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Article Engineering, Chemical

A novel Ag/PANI/ZnTiO3 ternary nanocomposite as a highly efficient visible-light-driven photocatalyst

M. Faisal et al.

Summary: The study successfully synthesized Ag and PANI doped ZnTiO3 ternary photocatalyst, demonstrating its high efficiency in environmental remediation. The formation of the novel ternary photocatalyst altered the bandgap energy of ZnTiO3 and exhibited excellent degradation performance under visible light illumination.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Environmental

N-doped magnetic three-dimensional carbon microspheres@TiO2 with a porous architecture for enhanced degradation of tetracycline and methyl orange via adsorption/photocatalysis synergy

Yushun Zhou et al.

Summary: A novel catalyst of N-doped magnetic three-dimensional (3D) carbon microspheres@TiO2 was developed from low-cost biomass of chitin, showing high surface area and excellent photocatalytic degradation performance.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Physical

Enhanced photocatalytic degradation of gaseous toluene and liquidus tetracycline by anatase/rutile titanium dioxide with heterophase junction derived from materials of Institut Lavoisier-125(Ti): Degradation pathway and mechanism studies

Xiaodong Zhang et al.

Summary: Anatase/rutile titanium dioxide with heterophase junction and large BET specific surface area was successfully synthesized by calcinating MIL-125(Ti) with 30% O-2/Ar at 600 degrees C. The photocatalytic performance of M-O-600 in degrading toluene and tetracycline under visible light illumination was significantly influenced by calcination temperature, with M-600 displaying outstanding activity.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Engineering, Environmental

Design of core-shelled g-C3N4@ZIF-8 photocatalyst with enhanced tetracycline adsorption for boosting photocatalytic degradation

Xin Yuan et al.

Summary: The study found that gC3N4@ZIF-8 exhibits superior performance in enhancing TC degradation, with significantly higher degradation rate constant and removal rate compared to gC3N4 alone. Additionally, the optimized material also shows excellent degradation and removal efficacy in RhB and Cr (VI), accelerating pollutant degradation by promoting the formation and transformation of oxygen radicals.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Engineering, Environmental

Strategies for improving perovskite photocatalysts reactivity for organic pollutants degradation: A review on recent progress

Kexin Wei et al.

Summary: This review summarizes recent progress in tuning strategies and coupling Advanced Oxidation Processes (AOPs) methods to improve perovskite photocatalyst reactivity for water decontamination. It introduces general principles of designing perovskite photocatalysts for water decontamination and discusses diverse strategies to enhance perovskite photocatalytic activity. Additionally, it presents the rapid development of coupling various AOPs with perovskite for improved water remediation and discusses remaining challenges and future directions for practical perovskite photocatalytic water purification.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Chemical

Fabrication of 3D Bi5O7I/BiOIO3 heterojunction material with enhanced photocatalytic activity towards tetracycline antibiotics

Zhijia Zhu et al.

Summary: The study successfully prepared Bi5O7I/BiOIO3 composite materials with excellent degradation efficiency and stability in photocatalysis. Through investigation of electron migration and photocatalytic mechanism, it elucidated the active species and heterojunction structure contributing to the improved photocatalytic activity.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Chemical

Removal of tetracycline hydrochloride in aqueous by coupling dielectric barrier discharge plasma with biochar

Jing Lou et al.

Summary: The study found that dielectric barrier discharge combined with biochars can effectively remove tetracycline hydrochloride in water, with BC600 showing the best removal performance. Increasing peak voltage and pH can enhance the removal efficiency of TCH, while ?OH and ?O2 ? are important pathways for removal. During the discharge plasma process, the specific surface areas and oxygen functional groups of BC600 increased, contributing to the higher removal efficiency.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Environmental

Visible-light-driven activation of peroxymonosulfate for accelerating ciprofloxacin degradation using CeO2/Co3O4 p-n heterojunction photocatalysts

Chun-Hui Shen et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Engineering, Environmental

Adsorption behavior of tetracycline from aqueous solution on ferroferric oxide nanoparticles assisted powdered activated carbon

Jiahui Zhou et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Engineering, Environmental

Enhancing rejection performance of tetracycline resistance genes by a TiO2/AgNPs-modified nanofiber forward osmosis membrane

Haisheng Chen et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Chemistry, Physical

Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance

Qijun Tang et al.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2020)

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Article Engineering, Environmental

Tetracycline removal by double-metal-crosslinked alginate/graphene hydrogels through an enhanced Fenton reaction

Yan Kong et al.

JOURNAL OF HAZARDOUS MATERIALS (2020)

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Review Environmental Sciences

A review on the preparation, characterization and potential application of perovskites as adsorbents for wastewater treatment

Zaharaddeen N. Garba et al.

CHEMOSPHERE (2020)

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Fabrication of novel CuFe2O4/MXene hierarchical heterostructures for enhanced photocatalytic degradation of sulfonamides under visible light

Yang Cao et al.

JOURNAL OF HAZARDOUS MATERIALS (2020)

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Novel CoS2/MoS2@Zeolite with excellent adsorption and photocatalytic performance for tetracycline removal in simulated wastewater

Junfei Liu et al.

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A review on MXene-based nanomaterials as adsorbents in aqueous solution

Minjung Jeon et al.

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Efficient reduction of Cr(VI) by a BMO/Bi2S3 heterojunction via synergistic adsorption and photocatalysis under visible light

Xueqing Li et al.

JOURNAL OF HAZARDOUS MATERIALS (2020)

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Adsorption and photocatalytic degradation mechanism of magnetic graphene oxide/ZnO nanocomposites for tetracycline contaminants

Disi Qiao et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Effective removal of Pb(ii) from synthetic wastewater using Ti3C2Tx MXene

Byung-Moon Jun et al.

ENVIRONMENTAL SCIENCE-WATER RESEARCH & TECHNOLOGY (2020)

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X-ray absorption spectroscopy analysis and photocatalytic behavior of ZnTiO3 nanoparticles doped with Co and Mn synthesized by sonochemical method

Chakkaphan Wattanawikkam et al.

APPLIED SURFACE SCIENCE (2019)

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Ferromagnetic Enhancement in ZnTiO3 films induced by Co doping

Yangjun Yan et al.

CERAMICS INTERNATIONAL (2019)

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Hydrogen adsorption-induced catalytic enhancement over Cu nanoparticles immobilized by layered Ti3C2 MXene

Lijun Liu et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Properties of two-dimensional Ti3C2 MXene/thermoplastic polyurethane nanocomposites with effective reinforcement via melt blending

Xinxin Sheng et al.

COMPOSITES SCIENCE AND TECHNOLOGY (2019)

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Removal of tetracycline from aqueous solution using Fe-doped zeolite

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INTERNATIONAL JOURNAL OF INDUSTRIAL CHEMISTRY (2019)

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Sustainable efficient adsorbent: Alkali-acid modified magnetic biochar derived from sewage sludge for aqueous organic contaminant removal

Lin Tang et al.

CHEMICAL ENGINEERING JOURNAL (2018)

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One-step synthesis of Co-doped UiO-66 nanoparticle with enhanced removal efficiency of tetracycline: Simultaneous adsorption and photocatalysis

Jiao Cao et al.

CHEMICAL ENGINEERING JOURNAL (2018)

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Controlled charge-dynamics in cobalt-doped TiO2 nanowire photoanodes for enhanced photoelectrochemical water splitting

Changhai Liu et al.

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Adsorptive performance of MOF nanocomposite for methylene blue and malachite green dyes: Kinetics, isotherm and mechanism

Ayoub Abdullah Alqadami et al.

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Adsorption of tetracycline antibiotics from aqueous solutions on nanocomposite multi-walled carbon nanotube functionalized MIL-53 (Fe) as new adsorbent

Weiping Xiong et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2018)

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Ag3PO4/Ti3C2 MXene interface materials as a Schottky catalyst with enhanced photocatalytic activities and anti-photocorrosion performance

Tao Cai et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2018)

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Synergy of adsorption and visible-light photocatalytic degradation of methylene blue by a bifunctional Z-scheme heterojunction of WO3/g-C3N4

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Theoretical study on the adsorption of carbon dioxide on individual and alkali-metal doped MOF-5s

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RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A (2016)

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In situ synthesis of In2S3@MIL-125(Ti) core-shell microparticle for the removal of tetracycline from wastewater by integrated adsorption and visible-light-driven photocatalysis

Hou Wang et al.

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A novel magnetic Fe@Au core-shell nanoparticles anchored graphene oxide recyclable nanocatalyst for the reduction of nitrophenol compounds

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Ag doped and Ag dispersed nano ZnTiO3: Improved photocatalytic organic pollutant degradation under solar irradiation and antibacterial activity

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Activated carbon supported cobalt catalysts for advanced oxidation of organic contaminants in aqueous solution

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APPLIED CATALYSIS B-ENVIRONMENTAL (2010)

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Adsorptive and photocatalytic performance of cobalt-doped ZnTiO3/Ti3C2Tx MXene nanohybrids towards tetracycline: Kinetics and mechanistic insight

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