Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 81, Issue 8, Pages 3065-3069Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.6b00587
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Funding
- Challenging Exploratory Research
- Ministry of Education, Culture, Sports, Science and Technology, Japan
- Grants-in-Aid for Scientific Research [16H04145, 15K13688] Funding Source: KAKEN
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An intermolecular three-component arylsilylation of alkynes has been developed under mild palladium/copper cooperative catalysis. The reaction proceeds through syn-addition of an aryl group and a silyl group across the carbon carbon triple bond of an alkyne. This represents the first transition-metal-catalyzed fully intermolecular arylsilylation of alkynes, and transformations of the resulting products have also been demonstrated.
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