Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume -, Issue -, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.202203334
Keywords
anodes; electrolytes; high voltage; interphase; magnesium metal batteries
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The demand for high-energy-density and safe energy storage devices has led to increased interest in high-voltage rechargeable magnesium batteries (RMB). The development of high-voltage electrolytes, which serve as the bridge between cathode and anode materials, is crucial for realizing high-voltage RMBs. This paper provides an overview of three chloride-free electrolyte systems with wide electrochemical windows, discusses degradation mechanisms and modification strategies at the anode/electrolyte interphase, and highlights future directions for stabilizing magnesium anodes and achieving high-voltage RMBs.
The demand for high-energy-density and safe energy storage devices has spurred increasing interest in high-voltage rechargeable magnesium batteries (RMB). As electrolytes are the bridge connecting the cathode and anode materials, the development of high-voltage electrolytes is the key factor in realizing high-voltage RMBs. This concept presents an overview of three chloride-free electrolyte systems with wide electrochemical windows, together with the degradation mechanisms and modification strategies at the anode/electrolyte interphase. Finally, future directions in stabilizing Mg anodes and realizing high-voltage RMBs are highlighted.
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