4.8 Review

Recent advances in conductive hydrogels: classifications, properties, and applications

Journal

CHEMICAL SOCIETY REVIEWS
Volume 52, Issue 2, Pages 473-509

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cs00173j

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This review explores the recent advances in multifunctional conductive hydrogels for electronic devices, including their different components and functionalities. The applications of hydrogels in flexible devices are illustrated, and the current challenges and future development prospects are discussed.
Hydrogel-based conductive materials for smart wearable devices have attracted increasing attention due to their excellent flexibility, versatility, and outstanding biocompatibility. This review presents the recent advances in multifunctional conductive hydrogels for electronic devices. First, conductive hydrogels with different components are discussed, including pure single network hydrogels based on conductive polymers, single network hydrogels with additional conductive additives (i.e., nanoparticles, nanowires, and nanosheets), double network hydrogels based on conductive polymers, and double network hydrogels with additional conductive additives. Second, conductive hydrogels with a variety of functionalities, including self-healing, super toughness, self-growing, adhesive, anti-swelling, antibacterial, structural color, hydrophobic, anti-freezing, shape memory and external stimulus responsiveness are introduced in detail. Third, the applications of hydrogels in flexible devices are illustrated (i.e., strain sensors, supercapacitors, touch panels, triboelectric nanogenerator, bioelectronic devices, and robot). Next, the current challenges facing hydrogels are summarized. Finally, an imaginative but reasonable outlook is given, which aims to drive further development in the future.

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