Journal
CATALYSIS COMMUNICATIONS
Volume 66, Issue -, Pages 10-14Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.catcom.2015.03.004
Keywords
g-C3N4; Chlorine modification; Photocatalytic zonation; Synergy
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Funding
- National Natural Science Foundation of China [21207133]
- National Science Fund for Distinguished Young Scholars of China [51425405]
- National Key Technology RD Program [2011BAC06B09]
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We coupled g-C3N4 or chlorine modified g-C3N4 (Cl/g-C3N4) photocatalysis with ozonation for mineralization of oxalic acid (OA) under visible light. g-C3N4 and Cl/g-C3N4 could trigger a super synergy between photocatalysis and ozonation, with a coupling coefficient at 17.8 and 9.9, respectively. The great gap of redox potential between the conduction band of g-C3N4 and ozone greatly benefitted electrons captured by ozone molecules, and thus promoted charge separation and ozone self-decomposition into a growing number of hydroxyl radicals in a photocatalytic ozonation process. Besides, the influence of chlorine modification on g-C3N4 to photocatalysis and photocatalytic ozonation was also clearly stated. (C) 2015 Elsevier B.V. All rights reserved.
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