A Covalent Organic Framework as a Long-life and High-Rate Anode Suitable for Both Aqueous Acidic and Alkaline Batteries

Article Chemistry, Multidisciplinary

A Symmetric All-Organic Proton Battery in Mild Electrolyte

Zhiwei Tie et al.

Summary: The design of all-organic proton batteries in mild electrolytes has been a challenge. In this study, a new molecule was designed and synthesized, allowing all-organic proton batteries to operate in a mild electrolyte.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

Stabilizing Interface pH by N-Modified Graphdiyne for Dendrite-Free and High-Rate Aqueous Zn-Ion Batteries

Qi Yang et al.

Summary: The study revealed the importance of interface pH in addressing the Zn dendrite issue. A novel N-modification graphdiyne interface (NGI) was constructed to stabilize pH and achieve dendrite-free Zn deposition, resulting in a significantly increased symmetric cell lifespan.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Physical

Advanced Pre-Diagnosis Method of Biomass Intermediates Toward High Energy Dual-Carbon Potassium-Ion Capacitor

Peng Cai et al.

Summary: A method for selecting biomass precursors and improving the structure of carbon materials to enhance the performance of potassium ion capacitors was proposed. The carbon materials obtained using this method as the battery-type anode exhibit high energy density and super high power output.

ADVANCED ENERGY MATERIALS (2022)

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Article Chemistry, Multidisciplinary

High-Voltage Organic Cathodes for Zinc-Ion Batteries through Electron Cloud and Solvation Structure Regulation

Huilin Cui et al.

Summary: This study explores the application of organic materials in zinc-ion batteries and successfully increases the output voltage of organic electrode by adjusting the energy change and manipulating the solvation structure.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Physical

Suppressed Dissolution and Enhanced Desolvation in Core-Shell MoO3@TiO2 Nanorods as a High-Rate and Long-Life Anode Material for Proton Batteries

Chenggang Wang et al.

Summary: This article investigates the application of MoO3 material in rechargeable proton batteries and suppresses material dissolution by coating a ultrathin TiO2 shell on MoO3 nanorods. The experimental results show that MoO3@TiO2 exhibits excellent electrochemical performance at high rates and high mass loadings.

ADVANCED ENERGY MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Designing Quinone-Based Anodes with Rapid Kinetics for Rechargeable Proton Batteries

Xinru Yang et al.

Summary: In this study, a series of quinone anodes were designed and studied, and it was discovered that tetramethylquinone exhibited high capacity, low polarization, and good capacity retention in acidic electrolyte. The study also revealed the mechanism of proton transport, providing important insights for the design of advanced aqueous batteries.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

Alkali-Durable Covalent Organic Frameworks Carrying In Situ Ammonium as an Ionic Conductor toward Hydroxide Transport

Bowen Yang et al.

Summary: In this study, a self-standing covalent organic framework (COF) membrane was synthesized and ionized to prepare an ionic conductor. The resulting ionic conductor exhibited excellent alkaline stability and high conductivity, making it suitable for applications such as water electrolysis, alkaline fuel cells, and hydrogen production.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2022)

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Article Chemistry, Physical

A significantly improved polymer∥Ni(OH)2 alkaline rechargeable battery using anthraquinone-based conjugated microporous polymer anode

Rebecca Grieco et al.

Summary: This study presents a novel polymer alkaline rechargeable battery (ARB) using a robust anthraquinone-based conjugated microporous polymer (IEP-11) as an anode. The IEP-11 parallel to Ni(OH)(2) exhibits high cell voltage, high capacities, long cycle life, excellent rate performance, and low temperature operativity in low concentrate electrolyte. It outperforms traditional linear poly (anthraquinone sulfide) (PAQS) and most reported organic parallel to nickel (Ni)/cobalt (Co)/manganese (Mn) ARBs.

MATERIALS TODAY ENERGY (2022)

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Article Chemistry, Physical

Advanced In Situ Induced Dual-Mechanism Heterointerface Towards Ultrastable Aqueous Rocking-Chair Zinc-Ion Batteries

Peng Cai et al.

Summary: An advanced dual-mechanism Na1.6TiS2/CuSe2 heterostructure anode with built-in electric fields has been successfully constructed for ultrastable aqueous rocking-chair zinc-ion batteries, demonstrating excellent electrochemical performance and cycling stability.

ADVANCED ENERGY MATERIALS (2022)

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Article Chemistry, Physical

Stable colloid-in-acid electrolytes for long life proton batteries

Haocheng Guo et al.

Summary: The emerging proton electrochemistry provides opportunities for future high-capacity and high-rate energy storage. However, the development of proton batteries is hindered by low working potentials of electrodes and poor cycle life of full cells. In this study, we demonstrate the formation of homogeneous and stable MnO2 colloids through Mn2+ electrolysis in H2SO4, and their application for achieving long life proton batteries.

NANO ENERGY (2022)

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Article Chemistry, Physical

A covalent organic framework for high-rate aqueous calcium-ion batteries

Linyuan Li et al.

Summary: Calcium-ion batteries (CIBs) can benefit from using covalent organic frameworks (COFs) as anode materials, as they provide high specific capacity and outstanding rate performance. The storage mechanism of pseudocapacitance behavior in COFs contributes to the remarkable rate performance. This study demonstrates the potential of COF materials as active host materials for CIBs.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Review Nanoscience & Nanotechnology

Non-metallic charge carriers for aqueous batteries

Guojin Liang et al.

Summary: Non-metallic charge carriers play a crucial role in aqueous batteries, offering improved performance and reduced manufacturing costs. Through insertion into electrode frameworks and serving as reversible redox centers, non-metallic charge carriers demonstrate superior performance compared to metallic counterparts.

NATURE REVIEWS MATERIALS (2021)

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Article Chemistry, Organic

Degradation of Organic Cations under Alkaline Conditions

Wei You et al.

Summary: Understanding the degradation mechanisms of organic cations under basic conditions is crucial for the development of durable alkaline energy conversion devices. An evaluation of 26 model compounds is being conducted to identify cations with improved alkaline stabilities and advance the field.

JOURNAL OF ORGANIC CHEMISTRY (2021)

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Review Chemistry, Physical

Strategies for the Stabilization of Zn Metal Anodes for Zn-Ion Batteries

Zhehan Yi et al.

Summary: Zinc-ion batteries are considered promising candidates for next-generation energy storage systems due to their high safety, resource availability, and environmental friendliness. However, the instability of the Zn metal anode has hindered their reliable deployment, and efforts have been made to overcome this through electrode structure design, interface modification, and electrolyte/separator optimization. Understanding and categorizing these strategies based on their intrinsic mechanisms are important for the development of novel Zn metal anodes for ZIBs.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

A crystalline dihydroxyanthraquinone anodic material for proton batteries

Juezhi Yu et al.

Summary: This study demonstrates the reversible intercalation and deintercalation of protons in crystalline 2,6-dihydroxyanthraquinone (DHAQ), which is utilized in a rechargeable proton battery system with high capacity retention rate. Furthermore, the morphology evolution from particulate DHAQ into centimeter-scale nanofibers is observed during battery cycling.

MATERIALS TODAY ENERGY (2021)

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Article Chemistry, Physical

Dramatic HER Suppression on Ag Electrodes via Molecular Films for Highly Selective CO2 to CO Reduction

Arnaud Thevenon et al.

Summary: Selective conversion of CO2 to CO with high Faradaic efficiencies (>99%) on planar silver electrodes was achieved using simple pyridinium-based additives, which form organic films altering CO2RR selectivity. Electrochemical kinetic and mechanistic data suggest that a hydrophobic organic layer inhibits hydrogen production selectively by limiting proton mass transport, while pointing to proton transfer as the rate-determining step instead of electron transfer for planar Ag electrodes.

ACS CATALYSIS (2021)

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Article Chemistry, Physical

Proton-filtering covalent organic frameworks with superior nitrogen penetration flux promote ambient ammonia synthesis

Sisi Liu et al.

Summary: By controlling the diffusion of reactants and using proton-filtering covalent organic frameworks, a highly selective and active nitrogen reduction was achieved in electrochemical ammonia synthesis. This strategy optimizes mass transfer and provides guidelines for practical green ammonia production.

NATURE CATALYSIS (2021)

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Article Chemistry, Physical

High-rate aqueous zinc-organic battery achieved by lowering HOMO/LUMO of organic cathode

Zhuolin Ye et al.

Summary: The study introduces a new cathode material HATN-3CN by lowering the HOMO/LUMO energy of aromatic Schiff base with strong electron-withdrawing and conjugating groups (-CN), demonstrating excellent rate capacity and cycle life, and revealing C=N moieties as active sites for charge storage.

ENERGY STORAGE MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Synthesis, Postsynthetic Modifications, and Applications of the First Quinoxaline-Based Covalent Organic Framework

Valerie A. Kuehl et al.

Summary: A new synthetic protocol for highly ordered two-dimensional nanoporous covalent organic frameworks (2D-COFs) based on a quinoxaline backbone is reported in this study. The quinoxaline framework allows for postsynthetic modification by incorporating two different chemical functionalities within the nanopores, including layer-to-layer cross-linking. Membranes fabricated using this new 2D-COF demonstrate highly selective separations and significant performance enhancement post cross-linking.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Molecular Engineering of Covalent Organic Framework Cathodes for Enhanced Zinc-Ion Batteries

Wenxi Wang et al.

Summary: Covalent organic frameworks (COFs) show promising performance as electrode materials for electrochemical storage, particularly in zinc-ion batteries, when the quinone group is introduced into their structure to enhance Zn2+ storage capability and increase average charge-discharge potential. This study highlights the importance of molecular engineering in improving the practical charge storage performance of COFs.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Molecular Tailoring of an n/p-type Phenothiazine Organic Scaffold for Zinc Batteries

Nan Wang et al.

Summary: This study introduces an organic compound containing both n-type and p-type redox moieties, demonstrating a hybrid charge storage mechanism that combines the advantages of n- and p-type reactions and compensates for their drawbacks, showing high voltage, capacity, long lifespan, and high power characteristics.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Engineering, Environmental

Exposing (001) crystal facet on the single crystalline fl-Ni(OH)2 quasi-nanocubes for aqueous Ni-Zn batteries

Tingting Chen et al.

Summary: A hydrothermal method was used to synthesize uniform single-crystal fl-Ni(OH)2 quasi-nanocubes for developing a stable aqueous Ni-Zn battery with good energy density. The nanosized fl-NQNCs enhanced the stability of the cathode and accelerated the charge transfer process. The battery exhibited excellent areal specific capacity, energy density, power density, and flexibility under bending.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Multidisciplinary

Hydroxide Anion Transport in Covalent Organic Frameworks

Shanshan Tao et al.

Summary: Designing and synthesizing anionic covalent organic frameworks has been shown to promote hydroxide anion transport, achieving exceptional conductivity compared to linear polymers and other porous frameworks. The study reveals that hydroxide anions transport via a proton-exchange hopping mechanism. These results open up new possibilities for designing framework materials for energy conversions.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Review Chemistry, Multidisciplinary

Bismuth-based Nanomaterials for Aqueous Alkaline Batteries: Recent Progress and Perspectives

Xuefeng Shang et al.

Summary: AABs, known for their cost-effectiveness, environmental benignity and high safety, have attracted widespread attention as the most promising stational energy storage system. Bismuth-based materials, with special advantages such as non-toxicity, low redox potential and high theoretical capacity, are potential anode candidates in AABs. This review outlines the structure of Bi based materials, their energy storage mechanism, application in AABs and provides perspectives on future anode design and innovation direction.

CHEMNANOMAT (2021)

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Article Chemistry, Physical

An extended carbonyl-rich conjugated polymer cathode for high-capacity lithium-ion batteries

Shibing Zheng et al.

Summary: This study developed a novel carbonyl-rich covalent organic polymer, PPh-PTO, with enhanced capacity and cycling performance in lithium-ion batteries, providing a promising strategy for designing high-energy materials for energy storage.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Physical

High-performance all-organic aqueous batteries based on a poly(imide) anode and poly(catechol) cathode

Nagaraj Patil et al.

Summary: Aqueous all-polymer batteries (AqPBs) are considered promising solutions for safe, sustainable, and high-performance energy storage applications. The development of such batteries, however, requires precise optimization of both electrodes and the electrolyte composition in order to maintain stable redox activity and deliver optimal voltage output. A specific AqPB system using a poly(imide) (PI) anode and poly(catechol) (PC) cathode has been shown to exhibit tunable cell voltage depending on the salt used in the aqueous electrolyte, achieving a maximum energy/power density of 80.6 W h kg(anode+cathode)(-1)/348 kW kg(anode+cathode)(-1) in Li+/H+, surpassing previously reported AqPB systems.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Proton Insertion Chemistry of a Zinc-Organic Battery

Zhiwei Tie et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Multidisciplinary Sciences

Nitrogen-rich covalent organic frameworks with multiple carbonyls for high-performance sodium batteries

Ruijuan Shi et al.

NATURE COMMUNICATIONS (2020)

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Article Chemistry, Physical

Integrating Multiredox Centers into One Framework for High-Performance Organic Li-Ion Battery Cathodes

Chunyu Cui et al.

ACS ENERGY LETTERS (2020)

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Article Chemistry, Physical

Solid-State Proton Battery Operated at Ultralow Temperature

Lei Yan et al.

ACS ENERGY LETTERS (2020)

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Correction Nanoscience & Nanotechnology

Differentiating Double-Layer, Pseudocapacitance, and Battery-like Mechanisms by Analyzing Impedance Measurements in Three Dimensions (vol 12, pg 14071, 2020)

Jesse S. Ko et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Atomic Engineering Catalyzed MnO2 Electrolysis Kinetics for a Hybrid Aqueous Battery with High Power and Energy Density

Dongliang Chao et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

Phenanthroline Covalent Organic Framework Electrodes for High-Performance Zinc-Ion Supercapattery

Wenxi Wang et al.

ACS ENERGY LETTERS (2020)

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Article Chemistry, Multidisciplinary

Architecting a Stable High-Energy Aqueous Al-Ion Battery

Chunshuang Yan et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Materials Science, Multidisciplinary

Moss-like nickel-cobalt phosphide nanostructures for highly flexible all-solid-state hybrid supercapacitors with excellent electrochemical performances

Guangmeng Qu et al.

APPLIED MATERIALS TODAY (2020)

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Article Chemistry, Physical

Phenazine anodes for ultralongcycle-life aqueous rechargeable batteries

Leilei Li et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Review Materials Science, Multidisciplinary

Chemically Robust Covalent Organic Frameworks: Progress and Perspective

Xinle Li et al.

MATTER (2020)

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Article Chemistry, Multidisciplinary

A High-Rate Two-Dimensional Polyarylimide Covalent Organic Framework Anode for Aqueous Zn-Ion Energy Storage Devices

Minghao Yu et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Review Chemistry, Multidisciplinary

Dendrites in Zn-Based Batteries

Qi Yang et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

High performance polyanthraquinone/Co-Ni(OH)2 aqueous batteries based on hydroxyl and potassium insertion/extraction reactions

Chang Liu et al.

SUSTAINABLE ENERGY & FUELS (2020)

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Article Engineering, Chemical

Tuning hydrogen bond and flexibility of N-spirocyclic cationic spacer for high performance anion exchange membranes

Yang Zhang et al.

JOURNAL OF MEMBRANE SCIENCE (2020)

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Article Chemistry, Multidisciplinary

Hierarchically hollow structured NiCo2S4@NiS for high-performance flexible hybrid supercapacitors

Guangmeng Qu et al.

NANOSCALE (2020)

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A Hollow Microtubular Triazine- and Benzobisoxazole-Based Covalent Organic Framework Presenting Sponge-Like Shells That Functions as a High-Performance Supercapacitor

Ahmed F. M. El-Mahdy et al.

CHEMISTRY-AN ASIAN JOURNAL (2019)

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Super-Stretchable Zinc Air Batteries Based on an Alkaline-Tolerant Dual-Network Hydrogel Electrolyte

Longtao Ma et al.

ADVANCED ENERGY MATERIALS (2019)

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Phenothiazine-Based Organic Catholyte for High-Capacity and Long-Life Aqueous Redox Flow Batteries

Changkun Zhang et al.

ADVANCED MATERIALS (2019)

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An Electrolytic Zn-MnO2 Battery for High-Voltage and Scalable Energy Storage

Dongliang Chao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Chemically stable polyarylether-based covalent organic frameworks

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NATURE CHEMISTRY (2019)

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A Pyrazine-Based Polymer for Fast-Charge Batteries

Minglei Mao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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A Nitrogen-Rich 2D sp2-Carbon-Linked Conjugated Polymer Framework as a High-Performance Cathode for Lithium-Ion Batteries

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Electrochemically activated spinel manganese oxide for rechargeable aqueous aluminum battery

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Direct synthesis of covalent triazine-based frameworks (CTFs) through aromatic nucleophilic substitution reactions

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RSC ADVANCES (2019)

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Zinc ion interactions in a two-dimensional covalent organic framework based aqueous zinc ion battery

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Controlling the strength of interaction between carbon dioxide and nitrogen-rich carbon materials by molecular design

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SUSTAINABLE ENERGY & FUELS (2019)

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MoS2 nanosheets with expanded interlayer spacing for rechargeable aqueous Zn-ion batteries

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ENERGY STORAGE MATERIALS (2019)

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Editorial Material Chemistry, Multidisciplinary

Energy Storage in Nanomaterials - Capacitive Pseudocapacitive, or Battery-like?

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Investigation of low-cost oligoanthraquinones for alkaline, aqueous rechargeable batteries with cell potential up to 1.13 V

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The Alkaline Stability of Anion Exchange Membrane for Fuel Cell Applications: The Effects of Alkaline Media

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Crystalline Dioxin-Linked Covalent Organic Frameworks from Irreversible Reactions

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Interlayer Hydrogen-Bonded Covalent Organic Frameworks as High-Performance Supercapacitors

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CHEM (2018)

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Review on the research of failure modes and mechanism for lead-acid batteries

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INTERNATIONAL JOURNAL OF ENERGY RESEARCH (2017)

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Advanced Organic Electrode Materials for Rechargeable Sodium-Ion Batteries

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Universal quinone electrodes for long cycle life aqueous rechargeable batteries

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The atom, the molecule, and the covalent organic framework

Christian S. Diercks et al.

SCIENCE (2017)

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Layered VS2 Nanosheet-Based Aqueous Zn Ion Battery Cathode

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Covalent organic frameworks based on Schiff-base chemistry: synthesis, properties and potential applications

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Reversible aqueous zinc/manganese oxide energy storage from conversion reactions

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NATURE ENERGY (2016)

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A high-capacity and long-life aqueous rechargeable zinc battery using a metal oxide intercalation cathode

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Hydroxide-ion induced degradation pathway for dimethylimidazolium groups in anion exchange membranes

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Covalent organic frameworks (COFs): from design to applications

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A Covalent Organic Framework as a Long-life and High-Rate Anode Suitable for Both Aqueous Acidic and Alkaline Batteries

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