4.5 Article

Caprock self-sealing effect due to CO2 leakage from geologic carbon sequestration reservoirs: a case study at Ping'an, China

Journal

FRONTIERS IN ENERGY RESEARCH
Volume 10, Issue -, Pages -

Publisher

FRONTIERS MEDIA SA
DOI: 10.3389/fenrg.2022.955465

Keywords

geological CO2 storage; CO2 leakage; self-sealing; travertin; Ping'an

Categories

Funding

  1. Qinghai Province Kunlun Talents Action Plan [2022-ZJ-735]
  2. High-level Talent Project of Bureau of Geological Exploration and Development of Qinghai Province [DD20221818]
  3. Qinghai Province Science and Technology Application Basic Research Project
  4. China Geological Survey Project
  5. [18]
  6. [16]

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Based on water quality test results and geological observation data, this study conducted numerical simulation and found that CO2-rich water migration towards the surface leads to the self-sealing effect of gypsum dissolution and calcite precipitation. This self-sealing effect forms rapidly and becomes more pronounced closer to the surface.
As a bottom technology for CO2 reduction, geological CO2 storage has attracted great attention from geologists, but there are few reports on the research of the caprock self-sealing effect due to CO2 leakage. Ping'an is a natural CO2 leakage site, which can be compared to the leakage scenarios of geological CO2 storage. Based on the water quality test results and geological observation data, the numerical simulation of geochemistry is carried out. The results show that: First, gypsum dissolves and calcite precipitates during the migration of CO2-rich water to the surface. This process presents a self-sealing effect, and the closer to the surface, the more obvious the self-sealing; Second, the self-sealing effect is formed rapidly. For a 30 cm wide fissure, it only takes a few hundred days to achieve self-sealing; Third, the CO2 leakage was estimated, about 140,813.3 m(3), or about 251.28 tons for 1 m long fissure.

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