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Recent status and future perspectives of 2D MXene for micro-supercapacitors and micro-batteries

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Flexible and high-performance electrochromic devices enabled by self-assembled 2D TiO2/MXene heterostructures

Ran Li et al.

Summary: Transition metal oxides (TMOs) are promising electrochromic (EC) materials for applications such as smart windows and displays, but achieving good flexibility, high coloration efficiency and fast response simultaneously remains a challenge. MXenes and their derived TMOs are good candidates for high-performance and flexible EC devices due to their 2D nature and the possibility of assembling them into loosely networked structures. The authors demonstrate flexible, fast, and high-coloration-efficiency EC devices based on self-assembled 2D TiO2/Ti3C2Tx heterostructures, with the Ti3C2Tx layer as the transparent electrode and the 2D TiO2 layer as the EC layer.

NATURE COMMUNICATIONS (2021)

Article Chemistry, Physical

Microsupercapacitor with a 500 nm gap between MXene/CNT electrodes

Eunji Kim et al.

Summary: This study presents a method for fabricating on-chip symmetric MSCs with coplanar interdigitated electrodes using focused-ion-beam process and carbon nanotube electrodes. The micro supercapacitors produced have high areal capacitance with narrow gaps between electrode fingers, while electron beam lithography and photolithography are utilized to create ultra-small footprint devices.

NANO ENERGY (2021)

Article Energy & Fuels

Recent progress on laser fabrication of on-chip microsupercapacitors

Xiaozhang Wang et al.

Summary: Laser direct writing technique proves its potential in producing high-performance microsupercapacitors through beam scanning, processing and patterning active substance simultaneously to form electrode features with high spatial resolution and accuracy. This method can construct 3D porous graphene, hierarchical porous frames, and nanostructures with precisely controlled porosity, facilitating the absorption, penetration, and transport of electrolyte ions for increased electrochemical performance in energy storage applications.

JOURNAL OF ENERGY STORAGE (2021)

Article Chemistry, Physical

Two-dimensional MXenes for electrochemical capacitor applications: Progress, challenges and perspectives

Qizhen Zhu et al.

Summary: MXenes, a family of 2D transition metal carbides/nitrides, show great potential for energy storage applications, with Ti3C2Tx being the most studied one. This review summarizes recent advances and challenges of MXenes for supercapacitors, discussing preparation methods, composition versatility, material architectures, and energy storage mechanisms. Future development of MXenes for designing next-generation supercapacitors is also provided.

ENERGY STORAGE MATERIALS (2021)

Article Nanoscience & Nanotechnology

Inkjet Printing Transparent and Conductive MXene (Ti3C2Tx) Films: A Strategy for Flexible Energy Storage Devices

Dong Wen et al.

Summary: In this study, a low-cost, large-scale, and rapid preparation method for flexible and transparent MXene films via inkjet printing was reported. The MXene films showed high sheet resistance and desirable transmittance, along with superior electrochemical performance in transparent supercapacitors. The convenient manufacturing process and excellent electrochemical properties of inkjet-printed flexible and transparent MXene films broaden the application horizon for flexible energy storage devices.

ACS APPLIED MATERIALS & INTERFACES (2021)

Review Materials Science, Multidisciplinary

Direct Ink Writing of Moldable Electrochemical Energy Storage Devices: Ongoing Progress, Challenges, and Prospects

Quanhai Zhang et al.

Summary: Direct ink writing (DIW) technology is extensively utilized in fabricating energy storage devices due to its excellent process flexibility and geometric controllability, offering higher power density and energy density compared to traditional casting techniques. Recent advances in DIW for emerging energy storage devices, such as SCs, lithium-ion batteries, lithium-sulfur batteries, rechargeable lithium metal batteries, and solid-state batteries, as well as the challenges and potential research possibilities are discussed. It is expected that with the development of 3D printing technology, batteries and SCs with durable lifespans, favorable safety, high energy density, and power density will be widely utilized in various fields.

ADVANCED ENGINEERING MATERIALS (2021)

Article Engineering, Chemical

Research progress on construction and energy storage performance of MXene heterostructures

Fanfan Liu et al.

Journal of Energy Chemistry (2021)

Review Chemistry, Analytical

Progress and Perspectives in Designing Flexible Microsupercapacitors

La Li et al.

Summary: This review discusses the recent progress in flexible microsupercapacitors and their applications in integrated wearable electronics, providing solutions to manufacturing, design, and integration requirements. It also considers guidelines for improving the electrochemical performance of flexible MSCs through materials design, device construction, and electrolyte optimization, and discusses the future challenges and prospects of flexible MSCs.

MICROMACHINES (2021)

Review Chemistry, Multidisciplinary

Electrical Conductivity Enhancement and Electronic Applications of 2D Ti3C2Tx MXene Materials

Chunyang Qiao et al.

Summary: This review highlights the recent progress on Ti3C2Tx MXene materials, focusing on their electrical performance and applications. Various aspects of enhancing the electrical conductivity of Ti3C2Tx MXene are carefully reviewed, providing a summary and discussing challenges for further improvement.

ADVANCED MATERIALS INTERFACES (2021)

Review Materials Science, Ceramics

From structural ceramics to 2D materials with multi-applications: A review on the development from MAX phases to MXenes

Aiguo Zhou et al.

Summary: MAX phases and MXenes are key focuses of research, with MAX phases known for their unique microstructure and properties, particularly their crack healing abilities; MXene research centers around preparation processes, microstructure, composites, and applications, with a primary focus on energy storage and electromagnetic interference shielding. New research directions and future trends on MAX phases and MXenes are also discussed.

JOURNAL OF ADVANCED CERAMICS (2021)

Review Chemistry, Physical

Spatial and Temporal Analysis of Sodium-Ion Batteries

Dewen Hou et al.

Summary: This Review summarizes significant recent progress in SIBs exploiting in situ and operando techniques based on X-ray and electron analyses at different time and length scales. Through the combination of spectroscopy, imaging, and diffraction, local and global changes in SIBs can be elucidated for improving materials design. The fundamental principles and state-of-the-art capabilities of different techniques are presented, followed by elaborative discussions of major challenges and perspectives.

ACS ENERGY LETTERS (2021)

Article Chemistry, Physical

Evolution and application of all-in-one electrochemical energy storage system

Ye Liu et al.

Summary: The review highlights the importance of all-in-one electrochemical energy storage devices in flexible electronics, discussing their fabrication strategies, performance, applications, and future challenges.

ENERGY STORAGE MATERIALS (2021)

Article Materials Science, Multidisciplinary

Materials and technologies for multifunctional, flexible or integrated supercapacitors and batteries

Wenbin Fu et al.

Summary: Electrochemical energy storage is crucial for portable medical and electronic devices, but traditional supercapacitors and batteries have limited integration capabilities. Future technologies will require batteries and hybrid devices that can seamlessly integrate into systems and adapt to various shapes, forms, and design functions.

MATERIALS TODAY (2021)

Review Multidisciplinary Sciences

Current advances and challenges in nanosheet-based wearable power supply devices

Sheng Zhang et al.

Summary: This article introduces the development and status of nanosheet-based wearable power supply devices, including nanosheet-based wearable batteries, supercapacitors, and self-powered energy suppliers. It also discusses the future opportunities and challenges of wearable devices.

ISCIENCE (2021)

Article Nanoscience & Nanotechnology

In-Situ Annealed Ti3C2Tx MXene Based All-Solid-State Flexible Zn-Ion Hybrid Micro Supercapacitor Array with Enhanced Stability

La Li et al.

Summary: Flexible Zn-ion hybrid micro-supercapacitors array using Ti3C2T as the cathode were fabricated via laser direct writing method and demonstrated excellent stability up to 50,000 cycles after in-situ annealed treatment. The potential application of the MSCs in integrated wearable electronics was highlighted by driving a digital timer and lighting a flexible LED displayer with the MSC arrays under different bending conditions.

NANO-MICRO LETTERS (2021)

Article Chemistry, Physical

Stencil-printed Lithium-ion micro batteries for IoT applications

Anju Toor et al.

Summary: The new micro lithium-ion battery design has high capacity for powering IoT devices, demonstrating significantly higher discharge capacity and energy density compared to other types of batteries, making it suitable for high peak current requirements in sensor systems.

NANO ENERGY (2021)

Review Electrochemistry

Strategies for Fabricating High-Performance Electrochemical Energy-Storage Devices by MXenes

LePing Yu et al.

Summary: MXenes, a unique family of materials, have been extensively studied for their applications in energy storage devices. This report provides a comprehensive overview of the synthesis methods, structural properties, as well as effective solutions to enhance the performance of energy storage devices using MXenes.

CHEMELECTROCHEM (2021)

Review Materials Science, Multidisciplinary

Direct Ink Writing of Materials for Electronics-Related Applications: A Mini Review

Zhenzhong Hou et al.

Summary: The fabrication of electronics-related components via direct ink writing (DIW) has attracted much attention recently due to the more complicated structures, higher accuracy, improved efficiency, and enhanced performances. DIW technology allows materials to be directly printed on a variety of flat substrates, making it suitable for applications such as wearable devices and on-chip integrations. The combination of DIW and electronic devices will help to improve the quality of human life and promote the development of science and society.

FRONTIERS IN MATERIALS (2021)

Review Chemistry, Multidisciplinary

Advances in Screen Printing of Conductive Nanomaterials for Stretchable Electronics

Nathan Zavanelli et al.

Summary: Stretchable electronics have shown great potential in various applications, but are limited by high-cost fabrication methods. Screen printing, with newly developed conductive nanomaterial inks, provides an exciting opportunity for scalable fabrication. The design of screen-printed inks is constrained by rheological requirements, substrate-ink attraction, and nanomaterial properties.

ACS OMEGA (2021)

Article Chemistry, Physical

Tunable capacitance in all-inkjet-printed nanosheet heterostructures

Yang Wang et al.

Summary: The research demonstrates the fabrication of supercapacitors based on 2D heterostructures using inkjet printing technology, showing high capacitance, good cycling stability, high energy and power densities, and potential for further improvement with the addition of liquid electrolytes.

ENERGY STORAGE MATERIALS (2021)

Article Chemistry, Physical

Electrostatic self-assembly of heterostructured black phosphorus-MXene nanocomposites for flexible microsupercapacitors with high rate performance

Jie Yang et al.

Summary: In this study, positively-charged black phosphorus (BP) nanoflakes were first prepared by electrochemical exfoliation method and electrostatically assembled with negatively-charged MXene nanosheets, forming heterostructured BP-MXene nanocomposites. Flexible BP-MXene thin films with lamellar structures and hierarchically porous networks were demonstrated, showing enhanced interfacial electron transfer. The flexible BP-MXene QMSC exhibited high volumetric energy density, outstanding rate performance, and high cyclability in neutral electrolytes, showcasing its potential as a promising flexible microscale power source for portable/wearable electronics.

ENERGY STORAGE MATERIALS (2021)

Article Nanoscience & Nanotechnology

Development and Applications of MXene-Based Functional Fibers

Si Qin et al.

Summary: This article highlights the recent exciting developments in research using MXene functionalized fibers, as well as the challenges that may be encountered in the processing. MXene, known for its metallic conductivity and high volumetric capacitance, holds promise for use in fibers and textile-based devices.

ACS APPLIED MATERIALS & INTERFACES (2021)

Review Chemistry, Multidisciplinary

Advances in the Synthesis of 2D MXenes

Yi Wei et al.

Summary: MXenes, versatile materials with adjustable structures and rich surface chemistry, have been recognized as potential 2D materials for various applications. Recent research has focused on synthetic routes, etching methods, and delamination strategies for large-scale preparation and stable storage. Antioxidation strategies for MXenes have also been summarized for future developments and practical applications.

ADVANCED MATERIALS (2021)

Article Chemistry, Multidisciplinary

Localized Water-In-Salt Electrolyte for Aqueous Lithium-Ion Batteries

Pauline Jaumaux et al.

Summary: A localized water-in-salt (LWIS) electrolyte based on low-cost lithium nitrate (LiNO3) salt and 1,5-pentanediol (PD) was developed, which improved electrolyte stability and cycling performance for aqueous Li-ion batteries. By in situ gelling the LWIS electrolyte with tetraethylene glycol diacrylate (TEGDA) monomer, the stability window was expanded to 3.0 V, resulting in excellent cycling performance with high Coulombic efficiency.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

Review Energy & Fuels

Recent Advances in Interface Engineering and Architecture Design of Air-Stable and Water-Resistant Lithium Metal Anodes

Yuanyuan Zhu et al.

Summary: This review discusses the importance of developing air-stable and waterproof lithium metal anodes for high-energy batteries, as well as the key strategies for suppressing the oxidation or corrosion of lithium metal anodes in air and water. It also examines current challenges and proposes future perspectives for the continuous development of air-stable and water-resistant lithium metal anodes.

ENERGY & FUELS (2021)

Review Energy & Fuels

Review on MXene synthesis, properties, and recent research exploring electrode architecture for supercapacitor applications

Arya Sohan et al.

Summary: This paper discusses the potential applications of MXenes in the field of supercapacitors, focusing on how their structure, properties, and surface chemistry impact energy storage, as well as the possibilities for improving supercapacitor performance through anode architecture based on MXenes. The review also emphasizes the selection of electrolytes and fabrication techniques for MXene-based anode fabrication, aiming to aid in future supercapacitor anode designing options.

INTERNATIONAL JOURNAL OF ENERGY RESEARCH (2021)

Review Materials Science, Multidisciplinary

3D-printed interdigital electrodes for electrochemical energy storage devices

Renpeng Chen et al.

Summary: This review discusses the advantages and progress in using 3D printing technology to manufacture interdigital electrochemical energy storage devices, explores the material requirements, and highlights recent research developments in 3D printing of electrodes for batteries and supercapacitors.

JOURNAL OF MATERIALS RESEARCH (2021)

Article Engineering, Electrical & Electronic

Advances in micro lithium-ion batteries for on-chip and wearable applications

Bingmeng Hu et al.

Summary: Miniature power sources, particularly micro lithium-ion batteries, have gained attention for their small size, lightweight, high capacity, and long cycle life, making them ideal for energy storage. Researchers have focused on optimizing performance and expanding applications, especially in on-chip integration and wearable applications.

JOURNAL OF MICROMECHANICS AND MICROENGINEERING (2021)

Article Chemistry, Physical

A flexible, heat-resistant and self-healable rocking-chair zinc ion microbattery based on MXene-TiS2 (de)intercalation anode

Bingtian Zhao et al.

Summary: A safe and environmentally friendly zinc ion microbattery with excellent electrochemical performance and self-healing properties has been developed, making it a feasible strategy for advanced high reliable and stable micro energy storage devices for wearable and integrated electronics.

JOURNAL OF POWER SOURCES (2021)

Review Electrochemistry

Review-Electrolyte and Electrode Designs for Enhanced Ion Transport Properties to Enable High Performance Lithium Batteries

Buket Boz et al.

Summary: This review focuses on studies investigating electrolyte and electrode designs to enhance ion transport properties for improved performance of LiBs. Efforts to enhance lithium transference number in organic electrolytes and significant ion transport challenges in porous electrodes are discussed. The review also highlights recent works on complex electrolytes and thick porous electrodes for high performance LiBs.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2021)

Review Chemistry, Applied

Electrospinning as a route to advanced carbon fibre materials for selected low-temperature electrochemical devices: A review

Yue Wen et al.

Summary: Electrospinning is a versatile method for producing nano-structured fibers with controllable morphology and surface properties, suitable for electrodes and flow media in various electrochemical devices, leading to efficiency improvements. The use of biomass as a polymer source has also gained attention for embedding sustainable principles in materials and increasing the use of renewable electricity.

JOURNAL OF ENERGY CHEMISTRY (2021)

Article Chemistry, Applied

Ink formulation, scalable applications and challenging perspectives of screen printing for emerging printed microelectronics

Ying Zhang et al.

Summary: Screen printing is a highly competitive manufacture technology for scalable and fast fabrication of printed microelectronics. Its large-scale application is limited by screen printing functional ink. This review summarizes recent advances, applications, and challenging perspectives of screen printing for emerging printed microelectronics.

JOURNAL OF ENERGY CHEMISTRY (2021)

Review Physics, Applied

Printed flexible supercapacitor: Ink formulation, printable electrode materials and applications

Jing Liang et al.

Summary: Flexible supercapacitors (FSCs) are attracting attention for their lightweight, easy integration, high power density, fast charge/discharge rate, and safety features. Printed FSC offers an economical solution for manufacturing, relying on functional inks formulation and innovative electrode materials design. The use of inks with excellent rheological properties and advanced electrode materials design are key to the success of next-generation printed FSC with high energy and high power.

APPLIED PHYSICS REVIEWS (2021)

Article Chemistry, Physical

Synchronously manipulating Zn2+ transfer and hydrogen/oxygen evolution kinetics in MXene host electrodes toward symmetric Zn-ions micro-supercapacitor with enhanced areal energy density

Zhiqia Cao et al.

Summary: The study presents a strategy to enhance Zn2+ diffusion and suppress hydrogen/oxygen evolution simultaneously within MXene host electrodes for high-energy-density symmetric ZMSCs. The designed MXene/BCF hybrid films effectively reduce Zn2+ diffusion barrier and induce additional pseudocapacitance, resulting in superior areal capacitance in ZMSCs. The use of a doubled voltage window in combination with suppressed kinetics of hydrogen/oxygen evolution leads to a significantly increased areal energy density compared to conventional electrolytes.

ENERGY STORAGE MATERIALS (2021)

Article Materials Science, Multidisciplinary

Synthesis of new two-dimensional titanium carbonitride Ti2C0.5N0.5Tx MXene and its performance as an electrode material for sodium-ion battery

Kun Liang et al.

Summary: A new 2D carbonitride MXene material, Ti2C0.5N0.5Tx, was reported in this study, showing higher specific capacities and larger electroactive surface area compared to traditional Ti2CTx powders. The multilayer Ti2C0.5N0.5Tx powders exhibited a specific capacity of 182 mAh g-1 at 20 mA g-1, the highest among reported MXene electrodes for SIBs, with excellent cycling stability.

INFOMAT (2021)

Review Chemistry, Multidisciplinary

Advances in wearable textile-based micro energy storage devices: structuring, application and perspective

Yixue Duan et al.

Summary: The continuous expansion of smart microelectronics has led to higher requirements for energy conversion, mechanical performance, and biocompatibility of micro-energy storage devices. Textile-based structures, with unique porosity, superior flexibility, and comfortable breathability, show great potential in wearable MESDs. This review comprehensively discusses the device construction, fabric processing, and smart functionalization of textile-based MESDs, as well as the perspectives on microfabrication processes and multiple applications of TMESDs.

NANOSCALE ADVANCES (2021)

Review Chemistry, Physical

Emerging Intercalation Cathode Materials for Multivalent Metal-Ion Batteries: Status and Challenges

Susu Chen et al.

Summary: Recent advances in intercalation cathode materials for multivalent metal-ion batteries, such as vanadium and manganese oxides, chalcogenides, and carbon materials, have shown promising potential. However, challenges remain in terms of sluggish solid-state diffusion and slow desolvation processes at the cathode/electrolyte interface.

SMALL STRUCTURES (2021)

Review Chemistry, Multidisciplinary

From bulk to interface: electrochemical phenomena and mechanism studies in batteries via electrochemical quartz crystal microbalance

Yuchen Ji et al.

Summary: EQCM technology is a powerful tool for understanding the bulk and interfacial behaviors during battery operation, enabling investigation into phenomena such as ion insertion/deinsertion, solid nucleation, and interphase formation. Recent studies have utilized EQCM to reveal phenomena and mechanisms in various batteries, showing promise for future applications in battery research.

CHEMICAL SOCIETY REVIEWS (2021)

Review Chemistry, Multidisciplinary

Ti3C2Tx MXene: from dispersions to multifunctional architectures for diverse applications

Ken Aldren S. Usman et al.

Summary: This review provides a comprehensive analysis of diverse solution-based processing methodologies for MXene-architecture fabrication and evaluates the processing challenges affecting material properties and device performance. Opportunities arising from these challenges are discussed to provide avenues for new designs in high performance applications.

MATERIALS HORIZONS (2021)

Review Chemistry, Multidisciplinary

High-voltage liquid electrolytes for Li batteries: progress and perspectives

Xiulin Fan et al.

Summary: The energy density of LIBs has been increased threefold since their introduction, but the capacity of transition metal oxide cathodes is approaching its limit due to stability limitations of electrolytes. To further enhance energy density, new high-capacity and high-voltage cathode materials need to be explored, and graphite anodes may need to be replaced. One of the main challenges for future development is the development of new electrolyte compositions that can accommodate high-voltage cathodes and anodes while ensuring the stability of the batteries.

CHEMICAL SOCIETY REVIEWS (2021)

Review Chemistry, Physical

Recent advancements in solid electrolytes integrated into all-solid-state 2D and 3D lithium-ion microbatteries

Albina Jetybayeva et al.

Summary: With the increasing significance of microelectronics and autonomous wireless devices in everyday life, the miniaturization of power sources has become a focal point of research. Solid-state Li-ion microbatteries are considered promising energy storage solutions, with LiPON electrolyte identified as a highly researched candidate.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

Article Materials Science, Multidisciplinary

Electronically coupled layered double hydroxide/MXene quantum dot metallic hybrids for high-performance flexible zinc-air batteries

Xiaotong Han et al.

Summary: The electronically and chemically coupled LDH/MQD/NG hybrids modulate the local electronic and surface structure of the active LDH, providing metallic conductivity and abundant active sites, leading to significantly improved bifunctional activity and electrocatalytic kinetics.

INFOMAT (2021)

Review Materials Science, Multidisciplinary

Laser irradiation construction of nanomaterials toward electrochemical energy storage and conversion: Ongoing progresses and challenges

Li Li et al.

Summary: This review comprehensively summarizes recent contributions and progress regarding laser-induced nanomaterials for ESCDs, with a special focus on their practical utilization in rechargeable batteries, supercapacitors and electrocatalysis. The discussion also includes detailed exploration of laser-induced synthesis strategies and mechanisms involved in nanoarchitecture generation/regulation, leading to optimized comprehensive performances of ESCDs.

INFOMAT (2021)

Review Chemistry, Physical

Recent advances in 2D MXenes: preparation, intercalation and applications in flexible devices

Jinxin Xu et al.

Summary: MXenes have gained much attention and developed rapidly since their discovery in 2011 due to their unique 2D structure and excellent properties. Various methods, from hazardous fluorine-based acid etching to safer routes like Lewis acid etching and chemical vapor deposition, have been successfully developed for preparing 2D MXenes. Intercalation or delamination is crucial for obtaining high-quality 2D MXene layers, and the flexibility, ductility, and stability of MXenes make them promising for applications in various fields.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

Article Nanoscience & Nanotechnology

Recent developments of stamped planar micro-supercapacitors: Materials, fabrication and perspectives

Fei Li et al.

Summary: This review discusses the recent progress in the development of stamping micro-supercapacitors, focusing on different materials and technologies. The manufacturing process and properties of each stamping method are scrutinized, along with technical difficulties and scientific challenges such as limited electrode thickness and poor printing resolution.

NANO MATERIALS SCIENCE (2021)

Article Nanoscience & Nanotechnology

Advanced architecture designs towards high-performance 3D microbatteries

Yang Li et al.

Summary: Rechargeable microbatteries are crucial for microelectronic devices, with high energy output and minimal footprint areas being key objectives. Besides new electrode materials, device configurations are also pivotal in enhancing performance and shrinking size. A revolutionary design based on rolled-up nanotechnology is important for achieving high energy output in a small footprint. Challenges and prospects in device design and materials optimization are discussed for future development.

NANO MATERIALS SCIENCE (2021)

Review Chemistry, Multidisciplinary

Smart fibers for energy conversion and storage

Wujun Ma et al.

Summary: Fibers have played a critical role in human development, particularly with the advancement of synthetic fibers making clothes stronger and more durable. The growth of smart and multifunctional fibers has been driven by the rise in miniature and wearable electronics. Advanced functional fibers for energy conversion and storage, such as nanogenerators and solar cells, are discussed, along with the importance of integrating fiber-shaped energy devices through smart structure design. Challenges and future directions in the field are highlighted, aiming to inspire scientists to contribute to the prosperity and development of smart fibers.

CHEMICAL SOCIETY REVIEWS (2021)

Review Chemistry, Multidisciplinary

Emerging trends in anion storage materials for the capacitive and hybrid energy storage and beyond

Qingyun Dou et al.

Summary: The article provides a comprehensive and systematic review of emerging anion storage materials in electrochemical and battery-capacitor hybrid devices, discussing their operating principles, classification, thermodynamic and kinetic aspects, as well as related interfaces. It also explores the charge storage mechanism, structure-property correlation, and electrochemical features of anion storage materials, along with recent progress in high-performance applications.

CHEMICAL SOCIETY REVIEWS (2021)

Review Chemistry, Physical

Ti3C2 MXene-polymer nanocomposites and their applications

Hossein Riazi et al.

Summary: MXene/polymer nanocomposites combine the strengths of MXenes and polymers, exhibiting superior properties in various engineering fields. This review critically examines the progress in these areas and identifies future research directions, including novel applications and surface modification approaches.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

Article Chemistry, Multidisciplinary

Ultrafast rechargeable Zn micro-batteries endowing a wearable solar charging system with high overall efficiency

Zhengnan Tian et al.

Summary: The study presents a wearable solar charging unit with high overall efficiency of 23.11%, based on a miniature GaAs solar cell and an ultrafast rechargeable Zn micro-battery. The system demonstrates favorable fast charging performance characteristics, providing continuous power supply for 110 s at 0.5 mA cm(-2) after 5 s of solar charging. By elucidating the electrochemical energy storage mechanism, the work offers an innovative strategy for constructing wearable solar charging units with advanced capabilities.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

Review Chemistry, Physical

3D printing-enabled advanced electrode architecture design

Tiankuo Chu et al.

Summary: This paper reviews recent studies on advanced electrode architecture design and manufacturing enabled by emerging additive manufacturing techniques for future high-performance energy storage devices. It highlights the importance of advanced electrode structure in promoting the performance of energy storage devices and summarizes the latest research on 3D printed electrodes.

CARBON ENERGY (2021)

Review Chemistry, Multidisciplinary

Ion regulation of ionic liquid electrolytes for supercapacitors

Jianze Feng et al.

Summary: As a member of the liquid electrolyte family, ionic liquids (ILs) are characterized by distinctive chemical and electrochemical stability, making them a promising candidate for high-performance supercapacitors (SCs). However, the high viscosity and poor ionic conductivity of ILs have hindered their rapid development in SC applications. One potential solution is ion regulation to modify IL electrolytes, leveraging the tunable nature of anions and cations. This paper provides an overview of recent advances in ion regulation for IL-based SCs, exploring the impact on energy storage mechanisms and electrochemical performance of electrode materials and devices. Additionally, it addresses the challenges and future directions for optimizing IL-based electrolytes in the next generation of SCs.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

Article Materials Science, Multidisciplinary

MXenes: An Emerging Platform for Wearable Electronics and Looking Beyond

Neng Li et al.

Summary: Wearable devices have potential applications in various fields, but the development of flexible wearable electronics is still in its early stages. MXenes, as wonder materials, have shown promise in energy storage and sensing applications across different research areas.

MATTER (2021)

Review Materials Science, Multidisciplinary

Three-dimensional printing of high-mass loading electrodes for energy storage applications

Hao Yang et al.

Summary: Nanostructured materials show great promise in energy storage applications due to their excellent electrochemical properties. However, traditional electrode fabrication methods limit the mass-loading, while 3D printing offers a solution to manufacture high-mass loading electrodes for improved electrochemical performance. This review discusses various 3D printing technologies and their applications in manufacturing high-mass loading electrodes for energy storage devices.

INFOMAT (2021)

Article Chemistry, Physical

Rolled-up island-bridge (RIB): a new and general electrode configuration design for a wire-shaped stretchable micro-supercapacitor array

Zhen Li et al.

Summary: A rolled-up island-bridge (RIB) architecture is demonstrated for fabricating a novel wire-shaped stretchable micro-supercapacitor array (WSS-MSCA) to achieve high energy density, large elongation, stable electrochemical output, and excellent integration capability and washability. The obtained WSS-MSCA can deliver a maximum linear/areal capacitance with high energy density and is able to function well under extreme deformations. This architecture guarantees outstanding integration capability of the MSC array, enabling on-demand output and ensuring unprecedented adjustability to the whole electrochemical performance of the device, making it a promising micro-power source for wearable microelectronics.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

Review Chemistry, Multidisciplinary

Recent advances in focused ion beam nanofabrication for nanostructures and devices: fundamentals and applications

Ping Li et al.

Summary: The article systematically summarizes and analyzes various factors related to FIB nanofabrication for the fabrication of 3D nanostructures and devices, including mechanisms, instruments, processes, and typical applications. Additionally, it highlights the current challenges and future development trends in the field of FIB nanofabrication.

NANOSCALE (2021)

Review Chemistry, Physical

Recent advances of hydrogel electrolytes in flexible energy storage devices

Cheuk Ying Chan et al.

Summary: Hydrogels, as promising electrolyte candidates, are regarded as the ideal choice for flexible energy storage devices due to their high-water absorbency and softness. By modifying chemical structures, diverse properties can be achieved, leading to the development of novel flexible energy storage devices with prolonged service life and unique functions.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

Article Chemistry, Multidisciplinary

Transfer Printing of Electronic Functions on Arbitrary Complex Surfaces

Jonghwa Park et al.

ACS NANO (2020)

Article Chemistry, Multidisciplinary

Ti3C2Tx MXene-Reduced Graphene Oxide Composite Electrodes for Stretchable Supercapacitors

Yihao Zhou et al.

ACS NANO (2020)

Article Materials Science, Multidisciplinary

Scalable Synthesis of Ti3C2Tx MXene

Christopher E. Shuck et al.

ADVANCED ENGINEERING MATERIALS (2020)

Article Materials Science, Multidisciplinary

Lithography and Etching-Free Microfabrication of Silicon Carbide on Insulator Using Direct UV Laser Ablation

Tuan-Khoa Nguyen et al.

ADVANCED ENGINEERING MATERIALS (2020)

Article Chemistry, Multidisciplinary

Substrate-Free and Shapeless Planar Micro-Supercapacitors

Pratteek Das et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

Review Chemistry, Physical

MXene/Polymer Membranes: Synthesis, Properties, and Emerging Applications

Lingfeng Gao et al.

CHEMISTRY OF MATERIALS (2020)

Review Optics

Parallel Laser Micro/Nano-Processing for Functional Device Fabrication

Yang Li et al.

LASER & PHOTONICS REVIEWS (2020)

Article Materials Science, Multidisciplinary

3D knitted energy storage textiles using MXene-coated yarns

Ariana Levitt et al.

MATERIALS TODAY (2020)

Review Physics, Multidisciplinary

Two-dimensional MXenes: From morphological to optical, electric, and magnetic properties and applications

Xiantao Jiang et al.

PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS (2020)

Article Nanoscience & Nanotechnology

Dual-Core Supercapacitor Yarns: An Enhanced Performance Consistency and Linear Power Density

Nanfei He et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

Article Chemistry, Multidisciplinary

MXene-Based Fibers, Yarns, and Fabrics for Wearable Energy Storage Devices

Ariana Levitt et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

Article Chemistry, Multidisciplinary

Turning Trash into Treasure: Additive Free MXene Sediment Inks for Screen-Printed Micro-Supercapacitors

Sina Abdolhosseinzadeh et al.

ADVANCED MATERIALS (2020)

Review Materials Science, Multidisciplinary

A review on MXene for energy storage application: effect of interlayer distance

Ruby Garg et al.

MATERIALS RESEARCH EXPRESS (2020)

Article Chemistry, Multidisciplinary

Additive-Free MXene Liquid Crystals and Fibers

Jizhen Zhang et al.

ACS CENTRAL SCIENCE (2020)

Article Nanoscience & Nanotechnology

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