Journal
ADVANCED MATERIALS INTERFACES
Volume 9, Issue 34, Pages -Publisher
WILEY
DOI: 10.1002/admi.202201248
Keywords
dissolution; interface instability; interfacial effect; moving contact line; wetting
Funding
- National Natural Science Foundation of China [12072346, 11722223]
- Chinese Academy of Sciences (CAS) Key Research Program of Frontier Sciences [QYZDJ-SSW-JSC019]
- Open Fund of Key Laboratory for Intelligent Nano Materials and Devices of the Ministry of Education [NJ2022002, INMD-2022M01]
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This paper presents a new type of instability called the pagoda instability (PI) that occurs when inserting a soluble fiber into a liquid. The coupling of dissolution and wetting leads to special phenomena and the final shapes of the fibers are summarized using a phase diagram. The use of optimized fibers can reduce the influence of capillary force during atomic force microscopy measurements in humid environments by 70%.
This paper presents a new kind of instability when inserting a soluble fiber into liquid. After wetting and dissolving the fiber by the liquid, the moving contact line (MCL) spontaneously loses stability. Because the sculpted shape of the fiber looks like a Chinese pagoda, this instability is named as the pagoda instability (PI). The coupling of dissolution and wetting leads to other special phenomena, i.e., dissolving-induced jet flow, and optimizes the fiber shape, etc. A criterion of PI is proposed and the competition between the interfacial energy and chemical potential to deduce the MCL motion and PI is shown. A phase diagram is used to summarize the final shapes of the fibers. By conducting atomic force microscopy (AFM) measurements, it is found that fibers with optimized shapes have a low adhesion force. Using the optimized fiber can decrease the influence of the capillary force during AFM measurements in humid environments by 70%.
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