4.7 Article

One-Dimensional Magnetic FeCoNi Alloy Toward Low-Frequency Electromagnetic Wave Absorption

Journal

NANO-MICRO LETTERS
Volume 14, Issue 1, Pages -

Publisher

SHANGHAI JIAO TONG UNIV PRESS
DOI: 10.1007/s40820-022-00920-7

Keywords

Medium-entropy magnetic alloy; One-dimension; Off-axis electronic holography technique; Improved electrospinning; Lower-frequency electromagnetic wave absorption

Funding

  1. National Natural Science Foundation of China [51725101, 11727807, 51672050, 61790581, 22088101]
  2. Ministry of Science and Technology of China (973 Project) [2018YFA0209102, 2021YFA1200600]
  3. Infrastructure and Facility Construction Project of Zhejiang Laboratory

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In this study, a composite EM wave absorber made of a FeCoNi medium-entropy alloy embedded in a 1D carbon matrix framework is rationally designed. The absorber shows high-density and continuous magnetic network and exhibits excellent magnetic loss ability. The enhanced EM wave absorption performance is mainly attributed to the 1D anisotropy and intrinsic physical features of the magnetic medium-entropy alloy.
Rational designing of one-dimensional (1D) magnetic alloy to facilitate electromagnetic (EM) wave attenuation capability in low-frequency (2-6 GHz) microwave absorption field is highly desired but remains a significant challenge. In this study, a composite EM wave absorber made of a FeCoNi medium-entropy alloy embedded in a 1D carbon matrix framework is rationally designed through an improved electrospinning method. The 1D-shaped FeCoNi alloy embedded composite demonstrates the high-density and continuous magnetic network using off-axis electronic holography technique, indicating the excellent magnetic loss ability under an external EM field. Then, the in-depth analysis shows that many factors, including 1D anisotropy and intrinsic physical features of the magnetic medium-entropy alloy, primarily contribute to the enhanced EM wave absorption performance. Therefore, the fabricated EM wave absorber shows an increasing effective absorption band of 1.3 GHz in the low-frequency electromagnetic field at an ultrathin thickness of 2 mm. Thus, this study opens up a new method for the design and preparation of high-performance 1D magnetic EM absorbers.

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