Journal
JOURNAL OF MATERIALS SCIENCE
Volume 52, Issue 9, Pages 4852-4865Publisher
SPRINGER
DOI: 10.1007/s10853-016-0720-z
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Funding
- National Natural Science Foundation of China [21373103]
- National Science and Technology Support Program [2014BAC03B06]
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Hollow urchin-like iron-doped manganese dioxide (Fe-MnO2) architectures were successfully prepared without any template or surfactant via a facile one-step hydrothermal route. Hollow urchin-like Fe-MnO2 architectures were made up of interleaving nanosheets, resulting in porous structures and high specific surface area. The formation mechanism of hollow urchin-like Fe-MnO2 architectures was proposed based on the Ostwald ripening process. When employed as supercapacitor electrode material, hollow urchin-like Fe-MnO2 delivered a specific capacitance of 203.3 F g(-1) at 250 mA g(-1) as well as a good capacity retention of 88.1% after 1000 cycles at 5 A g(-1). Coupled with activated carbon (AC) negative electrode, Fe-MnO2//AC asymmetric supercapacitor (Fe-MnO2//AC ASC) achieved an energy density of 20.2 Wh kg(-1) at a power density of 225 W kg(-1) and 83.8% capacity retention after 1000 cycles at 3 A g(-1), suggesting its potential applications for energy storage.
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