4.8 Article

Strong band renormalization and emergent ferromagnetism induced by electron-antiferromagnetic-magnon coupling

Journal

NATURE COMMUNICATIONS
Volume 13, Issue 1, Pages -

Publisher

NATURE PORTFOLIO
DOI: 10.1038/s41467-022-34254-0

Keywords

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Funding

  1. National Natural Science Foundation of China [11888101, 12074074, 11790312]
  2. National Key R&D Program of the MOST of China [2017YFA0303004, 2016YFA0300200]
  3. Shanghai Municipal Science and Technology Major Project [2019SHZDZX01]
  4. Shanghai Rising-Star Program [20QA1401400]
  5. DOE [DE-AC02-05CH11231]

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The interaction between antiferromagnetic magnons and electrons plays a crucial role in strongly correlated systems, directly influencing the band structure and properties of materials. The coupling constant of electron-antiferromagnetic magnon interactions can be significant, with strong dependence on doping and temperature. The colossal renormalization of electron bands by these interactions enhances the density of states at the Fermi energy, potentially leading to the emergence of new magnetic states in materials.
The interaction between antiferromagnetic magnons and electrons sits at the heart of many strongly correlated systems, however, investigation has been hampered by a lack of clear-cut examples. Here, Yu et al directly observe a kink in the dispersion, a result of renormalization due to the electron-antiferromagnetic magnon interaction. The interactions between electrons and antiferromagnetic magnons (AFMMs) are important for a large class of correlated materials. For example, they are the most plausible pairing glues in high-temperature superconductors, such as cuprates and iron-based superconductors. However, unlike electron-phonon interactions (EPIs), clear-cut observations regarding how electron-AFMM interactions (EAIs) affect the band structure are still lacking. Consequently, critical information on the EAIs, such as its strength and doping dependence, remains elusive. Here we directly observe that EAIs induce a kink structure in the band dispersion of Ba1-xKxMn2As2, and subsequently unveil several key characteristics of EAIs. We found that the coupling constant of EAIs can be as large as 5.4, and it shows strong doping dependence and temperature dependence, all in stark contrast to the behaviors of EPIs. The colossal renormalization of electron bands by EAIs enhances the density of states at Fermi energy, which is likely driving the emergent ferromagnetic state in Ba1-xKxMn2As2 through a Stoner-like mechanism with mixed itinerant-local character. Our results expand the current knowledge of EAIs, which may facilitate the further understanding of many correlated materials where EAIs play a critical role.

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