4.6 Article

The properties of silicate glass specimens for photon, neutron, and charged particles shielding: The roles of Bi2O3

Journal

RADIATION PHYSICS AND CHEMISTRY
Volume 201, Issue -, Pages -

Publisher

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.radphyschem.2022.110385

Keywords

Radiation shielding properties; Compton scattering technique; Neutron and charged particles; SRIM code

Funding

  1. Thailand Research Fund through the Research and Researchers for Industries (RRI) [PHD61I0013]
  2. NUCLEAR SYSTEM CO.,LTD
  3. National Research Council of Thailand (NRCT)
  4. Thailand Science Research and Innovation (TSRI)
  5. Chiang Mai University

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This experimental research aimed to study the shielding properties of glass specimens for photons, neutrons, and charged particles. The results showed that density and molar volume increased, and non-bridging oxygen (NBO) was generated in the glass structure. The mass attenuation coefficient (MAC), effective atomic number (Z(eff)), and effective electron density (N-eff) decreased with increasing energy, depending on the concentration of Bi(2)O(3). The half-value layer (HVL) and tenth-value layer (TVL) were thinner in the radiation shielding ability compared to other materials. The energy absorption buildup factor (EABF) and exposure buildup factor (EBF) depended on penetration depth and energy range. The total mass stopping power (TMSP) and projected range (PR) were calculated for charged particles shielding properties, and the fast neutron removal cross-section (FNRCS) was also calculated.
This experimental research aimed to study the photons, neutrons, and charged particles shielding properties of the glass specimens in the ratios xBi(2)O(3): 5Li(2)O: 20ZnO: (75-x)SiO2 where; x = 20, 25, 30, and 35 mol%. The specimens have been synthesized by the melt-quenching technique at 1200 ?. The WinXCom program used to compute the theoretical values of the mass attenuation coefficient (MAC). The Compton scattering technique is employed to be in the experiment for comparing the theoretical values in the energy range 0.225 MeV-0.662 MeV from the Cs-137 source. The result found that density and molar volume similarly increase and created non -bridging oxygen (NBO) in glass structure. The MAC, effective atomic number (Z(eff)), and effective electron density (N-eff) similarly abated with energy aggrandized and depended on the Bi(2)O(3 )concentrations. The half-value layer (HVL) and tenth-value layer (TVL) showed less thickness than other materials in the radiation shielding ability. The energy absorption buildup factor (EABF) and exposure buildup factor (EBF) are the same trends and depend on the penetration depth and energy range. The total mass stopping power (TMSP) and projected range (PR) have been reported using the SRIM program for charged particles shielding properties, and also concluded to calculate the fast neutron removal cross-section (FNRCS).

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