Journal
ORGANIC LETTERS
Volume -, Issue -, Pages -Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.2c02446
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- PAPIIT-DGAPA [IN208719, IN215322]
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A short strategy involving radical addition/cyclization cascade reaction and Pd-mediated cyclization was employed to synthesize three representative alkaloids of the (+/-)-rhazinilam family and 10 non-natural analogs.
A short, modular strategy for synthesizing three representative alkaloids of the (+/-)-rhazinilam family and 10 non-natural analogs is described. The protocol involves a radical addition/cyclization cascade reaction that assembles the tetrahydroindolizine system decorated with appropriate groups for a subsequent Pd-mediated cyclization, which generates the nine-membered lactam.
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