Journal
MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING
Volume 150, Issue -, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.mssp.2022.106944
Keywords
Thermoelectric material; Figure of merit; Nanostructuring; Thermal conductivity; Metamaterial
Categories
Funding
- Ministry of Science and Technology (Taiwan, R.O.C.) [MOST 109-2221-E-009-057-MY2]
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Thermoelectric materials play an important role in converting waste heat into useful electrical energy. Researchers have developed new mechanisms and strategies to optimize their performance in recovering low-grade heat. Balancing different thermoelectric parameters and focusing on lattice thermal conductivity can optimize the figure of merit (ZT) value. Band engineering, hierarchical scattering, and low-dimensionality techniques can enhance the power factor and reduce thermal conductivity. The synthesis of thermoelectric metamaterials may revolutionize the field by achieving a ZT value of 3.0.
Thermoelectric materials have been recognized as promising materials and make a prime contribution to con-verting waste heat into useful electrical energy without any further loss. In recent decades, researchers have witnessed the development of new and efficient mechanisms/strategies to optimize the figure of merit of these materials to recover the low-grade heat more efficiently. A balanced trade-off between TE parameters is indis-pensable to optimizing the ZT value. To some extent, the hit and trial method can be effective to optimize the TE properties. In electronic band engineering; the band convergence, the curvedness of the bandgap, or effective mass manipulation, significantly optimizes the power factor. Similarly, hierarchical scattering and low -dimensionality techniques are effective strategies to reduce thermal conductivity. It is better to pay more attention to the lattice thermal conductivity part rather than other TE properties to optimize the ZT value. For this one of the approaches is the introduction of various scales of defects in the specimen which scatter the phonons of all wavelengths. Finally, the notion of synthesizing TE metamaterials might bring a revolution in the TE materials system by mounting the ZT value to the threshold of 3.0.
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