Journal
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 13, Issue 37, Pages 8699-8710Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.2c02464
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The use of carbon nanotubes (CNTs) as electrocatalysts is analyzed in this paper. The limitations of using voltammetry based on CNT-modified electrodes are explained, and the role of mass transport and electrode kinetics in dictating the voltammetric responses is discussed. The paper advocates for the use of single-entity electrochemistry as a complement or potential replacement for ensemble voltammetry, emphasizing the importance of purity in CNT voltammetry.
The use of carbon nanotubes (CNTs) as electrocatalysts is summarized; the limitations of using voltammetry based on CNT-modified electrodes is explained; and the role of mass transport, as well as electrode kinetics, with respect to dictating the voltammetric responses is discussed. The use of single-entity electrochemistry to at least complement, if not replace, ensemble voltammetry is advocated along with other caveats, notably purity, with respect to CNT voltammetry.
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