4.7 Article

Silicon-coated fibrous network of carbon nanotube/iron towards stable and wideband electromagnetic wave absorption

Journal

JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
Volume 121, Issue -, Pages 199-206

Publisher

JOURNAL MATER SCI TECHNOL
DOI: 10.1016/j.jmst.2022.03.002

Keywords

Fibrous network; Silicon-coated nanostructure; Electromagnetic pollution; Magnetic-dielectric loss

Funding

  1. Ohio State University (OSU)
  2. OSU Institute for Materials Research Kickstart Facility Grant
  3. National Natural Science Foundation of China [31971740]
  4. Science and technology project of Jiangsu Province [BE2018391]
  5. Henan University of Science and technology
  6. OSU Sustainability Institute Seed Grant

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This study presents the design of fibrous nanostructures consisting of magnetic iron nanoparticles and carbon nanotubes for efficient and wide-band electromagnetic absorption. The nanostructures were coated with solid-state silicon to enhance stability and corrosion resistance. The research provides new avenues for utilizing electromagnetic absorbers in real-world applications such as anti-acid and oxidation ability.
Materials that can absorb electromagnetic (EM) wave have garnered increased attention in recent years due to their potential to mitigate the ever increasing environmental pollution by EM waves. Thanks to recent advances in micro/nanofabrication, a variety of magnetic metal-based EM absorbers have been reported. The design and synthesis of EM absorbers that exhibit efficient and wide-band absorption at small thicknesses, however, remains elusive. Here we report the design of fibrous nanostructures consisting of magnetic iron (Fe) nanoparticles and carbon nanotubes (CNTs), which exhibits a wide-band EM absorption (3.8 GHz) while maintain the thickness at 1.2 mm. In our work, we created a novel core-shell structure by immersing the highly fibrous CNT -Fe structure into solid-state silicon (SiO 2 ) matrix. Finally, the SiO 2 -coated CNT -Fe structures exhibit good stability against air-induced oxidation and acid corrosion while maintaining high EM absorption. Overall, the results reported in this study present new avenues to absorb EM from ambient air. We believe that our work elevates the utility of EM absorbers to real-world applications such as anti-acid and oxidation ability. (c) 2022 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology.

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