4.2 Article

Significant emission reductions of carbonaceous aerosols from residential coal burning by a novel stove

Journal

JOURNAL OF ENVIRONMENTAL SCIENCES
Volume 120, Issue -, Pages 135-143

Publisher

SCIENCE PRESS
DOI: 10.1016/j.jes.2021.08.042

Keywords

OC; EC; WSOC; Emission factor; Light absorption

Funding

  1. National Natural Science Foundation of China [21876186, 41727805, 41975164]
  2. National Research Program of Key Issues in Air Pollution Control [DQGG0206, DQGG0103, DQGG0209]

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This study developed a new household stove (NHS) to reduce the emissions of carbonaceous aerosols (CA). Compared with the traditional household stove (THS) under actual stove operation conditions, the NHS significantly reduced the emissions of OC, EC, and WSOC, as well as the mass absorption efficiency and radiative forcing of WSOC relative to EC.
Carbonaceous aerosols (CA) are crucial components in the atmospheric PM 2.5 and derived from diverse sources. One of the major sources for CA is from the incomplete combustion of bituminous coal that has been prevailingly used by household stoves in rural areas for heating during winter. To efficiently eliminate the CA emission, a new household stove (NHS) was developed based on a novel combustion technology and CA emissions from the NHS and a traditional household stove (THS) were comparably investigated under the actual stove operation conditions in a farmer???s house. Compared with the THS, the emission factors of organic carbon (OC), elemental carbon (EC), and water-soluble organic carbon (WSOC) from the NHS were reduced by 96% ??1%, 98% ??1%, and 91% ??1% under the flaming process and 95% ??1%, 96% ??2%, and 83% ??4% under the smoldering process, respectively. Additionally, the mass absorption efficiency of WSOC from the NHS reduced by 3 folds and the radiative forcing by WSOC relative to EC shrank remarkably by a factor of 3-8. Based on the reduction of emissions and light absorption of WSOC, the promotion of the NHS offers a possible solution to achieve the clean combustion of residential solid fuel. ?? 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.

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