4.7 Article

Lead isotopic compositions of late Archean lower continental crust

Journal

GEOCHIMICA ET COSMOCHIMICA ACTA
Volume 337, Issue -, Pages 95-105

Publisher

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.gca.2022.09.024

Keywords

Pb paradox; Granulite terrain; Granulite xenolith; Lower crust

Funding

  1. National Natural Science Foundation of China [41890832, 41973034, 41890833]

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The lead isotopes of Earth's silicate rocks pose a problem known as the first Pb paradox, as they are too radiogenic to have formed from meteoritic material. In this study, researchers investigate inaccessible rocks in order to find an unradiogenic reservoir that can balance Earth's bulk composition. By analyzing granulite terrain, granulite xenoliths, and lower crustal-derived granitoids from the northern North China craton, the researchers find that the late Archean lower crust may not be as extremely unradiogenic in Pb isotopic compositions as previously thought, and it appears insufficient to balance the accessible Earth.
Lead isotopes of Earth's accessible silicate rocks are generally too radiogenic for the planet to have formed from meteoritic material-a problem known as the first Pb paradox. The search for an unradiogenic reservoir to balance Earth's bulk composition has thus focused, with varying degrees of success, on inaccessible rocks in the core, mantle, and lower crust. Whether the lower continental crust balances the radiogenic depleted mantle and upper crust is debated and largely depends on how unradiogenic the lower crust, in particular the Archean lower crust, is. In this work, granulite terrain, granulite xenoliths, and lower crustal-derived granitoids from the same region of the northern North China craton (NCC) are combined to constrain the Pb isotopic compositions of the late Archean lower crust. The Hannuoba pyroxene-rich mafic granulite xenoliths are interpreted as restites left after partial melting of the late Archean lower crust to produce the Mesozoic granitoids. Both the xenoliths and granitoids have similar Pb isotopic compositions that are much more radiogenic than the granulite facies gneisses from the Huai'an terrain. The results rule out the notion that the lower crust is inherently poor in U and Th relative to Pb and suggest that the Pb isotopic compositions of the granulite facies gneisses are not representative of the Archean lower crust. This rule may be generally applicable to other regions because the Huai'an terrain is chemically and isotopically comparable with several other Archean unradiogenic granulite ter-rains (e.g., the Lewisian). We argue that the late Archean lower crust may not be so extremely unradio-genic in Pb isotopic compositions as commonly thought and the lower crust appears insufficiently unradiogenic to balance the accessible Earth. We also provide evidence that intracrustal differentiation via lower crustal melting could be an important mechanism causing the elevated Th/U and 208Pb/206Pb in the upper crust. (C) 2022 Elsevier Ltd. All rights reserved.

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