Journal
CATALYSIS TODAY
Volume 423, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.cattod.2022.08.016
Keywords
Nitrogen; Ammonia; Looping; Nitride; Mars-van Krevelen
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This article provides an overview of recent research on the possible involvement of the Mars-van Krevelen mechanism in ammonia synthesis catalyzed by metal nitrides, as well as literature on the synthesis of ammonia via chemical looping approaches.
Whilst the Mars-van Krevelen mechanism is well established for metal oxide catalysed oxidation reactions, it has been much less studied in the case of nitrogen based reactions catalysed by metal nitrides. In this overview, some of the recent literature in relation to the possible operation of the Mars- van Krevelen mechanism for ammonia synthesis catalysed by metal nitrides is presented, along with some of the literature relating to the synthesis of ammonia via chemical looping approaches.
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