Journal
ANNALS OF PHYSICS
Volume 447, Issue -, Pages -Publisher
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.aop.2022.169117
Keywords
Rare-Earth Iron Garnet; Magnetic Anisotropy; Magnetic Order; Ferrimagnetism; Chirality; Spintronics
Categories
Funding
- ICC-IMR
- Tohoku University
- QuantEmX grant from ICAM
- Gordon and Betty Moore Foundation [GBMF5305]
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Rare-earth iron garnets are important materials for spintronic devices. This study investigates the formation mechanism of umbrella-like spin structures in these garnets and explores the polarized spin wave dynamics. The findings improve the understanding of non-collinear magnetic phases in rare-earth iron garnets.
Rare-earth iron garnets R3Fe5O12 are fascinating insulators with very diverse magnetic phases. Their strong potential in spintronic devices has encouraged a renewal of interest in the study of their low temperature spin structures and spin wave dynamics. A striking feature of rare-earth garnets with R-ions exhibiting strong crystal-field effects like Tb-, Dy-, Ho-, Er-, Tm-and Yb-ions is the observation of low-temperature non-collinear magnetic structures featuring umbrella-likearrangements of the rare -earth magnetic moments. In this study, we demonstrate that such umbrella magnetic states are naturally emerging from the crystal-field anisotropies of the rare-earth ions. By means of a general model endowed with only the necessary elements from the crystal structure, we show how umbrella-like spin structures can take place and calculate the canting-angle as a result of the competition between the exchange-interaction of the rare-earth and the iron ions as well as the crystal-field anisotropy. Our results are compared to experimental data, and a study of the polarised spin wave dynamics is presented. Our study improves the understanding of umbrella-like spin structures and paves the way for more complex spin wave calculations in rare-earth iron garnets with non-collinear magnetic phases.(c) 2022 Elsevier Inc. All rights reserved.
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