Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 62, Issue 6, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202212857
Keywords
2D Materials; Covalent Functionalization; Graphene; Surface Chemistry
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This article reviews the latest advances in the covalent modification of supported graphene on substrates and focuses on analyzing different chemical modification methods, especially radical reactions. The study also reviews the recent achievements in reactivity control, tailoring electronic properties, and introducing active functionalities, and extends the analysis to other emerging 2D materials supported on surfaces.
In the last decade, the use of graphene supported on solid surfaces has broadened its scope and applications, and graphene has acquire a promising role as a major component of high-performance electronic devices. In this context, the chemical modification of graphene has become essential. In particular, covalent modification offers key benefits, including controllability, stability, and the facility to be integrated into manufacturing operations. In this Review, we critically comment on the latest advances in the covalent modification of supported graphene on substrates. We analyze the different chemical modifications with special attention to radical reactions. In this context, we review the latest achievements in reactivity control, tailoring electronic properties, and introducing active functionalities. Finally, we extended our analysis to other emerging 2D materials supported on surfaces, such as transition metal dichalcogenides, transition metal oxides, and elemental analogs of graphene.
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