4.8 Article

Colossal Room-Temperature Terahertz Topological Response in Type-II Weyl Semimetal NbIrTe4

Journal

ADVANCED MATERIALS
Volume 34, Issue 42, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202204621

Keywords

anisotropy; terahertz detectors; type-II Weyl semimetals

Funding

  1. National Key Research and Development Program of China [2021YFE0194200, 2021YFA1200903]
  2. National Natural Science Foundation of China [22175203, 22006023, 11974435]
  3. Natural Science Foundation of Guangdong Province [2019A1515010428, 2020A1515110821]
  4. Guangzhou Science and technology project [202102020126]
  5. Sichuan Natural Science Foundation [2022NSFSC1193]
  6. Plan Fostering Project of State Key Laboratory of Optoelectronic Materials and Technologies, of Sun Yat-sen University [OEMT2021-PZ-02]
  7. Nanyang Technological University Presidential Postdoctoral Fellowship

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This study fabricates a THz detector using a type-II Weyl semimetal (NbIrTe4), which shows excellent THz-detection performance due to the large tilting angle of Weyl nodes that improves photoresponsivity and mobility. The device also exhibits a giant intrinsic anisotropic conductance and THz response, both of which are record values.
The electromagnetic spectrum between microwave and infrared light is termed the terahertz (THz) gap, of which there is an urgent lack of feasible and efficient room-temperature (RT) THz detectors. Type-II Weyl semimetals (WSMs) have been predicted to host significant RT topological photoresponses in low-frequency regions, especially in the THz gap, well addressing the shortcomings of THz detectors. However, such devices have not been experimentally realized yet. Herein, a type-II WSM (NbIrTe4) is selected to fabricate THz detector, which exhibits a photoresponsivity of 5.7 x 10(4) V W-1 and a one-year air stability at RT. Such excellent THz-detection performance can be attributed to the topological effect of type-II WSM in which the effective mass of photogenerated electrons can be reduced by the large tilting angle of Weyl nodes to further improve mobility and photoresponsivity. Impressively, this device shows a giant intrinsic anisotropic conductance (sigma(max)/sigma(min) = 339) and THz response (Iph-max/Iph-min = 40.9), both of which are record values known. The findings open a new avenue for the realization of uncooled and highly sensitive THz detectors by exploring type-II WSM-based devices.

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