4.8 Article

All-Optical Tunability of Metalenses Permeated with Liquid Crystals

Journal

ACS NANO
Volume 16, Issue 10, Pages 16539-16548

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsnano.2c05887

Keywords

metalens; metasurface; reconfigurable; thermoplasmonics; liquid crystal; tunable

Funding

  1. Ohio Third Frontier Project Research Cluster on Surfaces in Advanced Materials (RC-SAM) at Case Western Reserve University
  2. NSF [1904592, FA9550-21-1-0312]
  3. AIM: Attraction and International Mobility PON R&I 2014-2020 Calabria
  4. Dottorati innovativi a caratterizzazione industriale PON R&I FSE-FESR 2014-2020
  5. NLHT -Nanoscience Laboratory for Human Technologies (POR Calabria FESR-FSE 14/20)
  6. A*STAR Singapore through the National Science Scholarship Scheme
  7. AFOSR MURI [NNCI-1542081]
  8. National Science Foundation under NSF award [ECCS-2025158]
  9. Direct For Mathematical & Physical Scien
  10. Division Of Chemistry [1904592] Funding Source: National Science Foundation

Ask authors/readers for more resources

In this paper, a nanostructured planar-fused silica metalens permeated with a nematic liquid crystal (NLC) and gold nanoparticle solution is presented. The embedded NLCs can be manipulated with external stimuli, enabling reconfigurable optical metasurfaces. The all-optical, dynamic control of the metalens optical response is achieved through thermoplasmonic-induced changes of the NLC solution associated with the nematic-isotropic phase transition.
Metasurfaces have been extensively engineered to produce a wide range of optical phenomena, allowing exceptional control over the propagation of light. However, they are generally designed as single-purpose devices without a modifiable postfabrica-tion optical response, which can be a limitation to real-world applications. In this work, we report a nanostructured planar-fused silica metalens permeated with a nematic liquid crystal (NLC) and gold nanoparticle solution. The physical properties of embedded NLCs can be manipulated with the application of external stimuli, enabling reconfigurable optical metasurfaces. We report the all-optical, dynamic control of the metalens optical response resulting from thermoplasmonic-induced changes of the NLC solution associated with the nematic-isotropic phase transition. A continuous and reversible tuning of the metalens focal length is experimentally demonstrated, with a variation of 80 mu m (0.16% of the 5 cm nominal focal length) along the optical axis. This is achieved without direct mechanical or electrical manipulation of the device. The reconfigurable properties are compared with corroborating numerical simulations of the focal length shift and exhibit close correspondence.

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