4.6 Article

Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield

Journal

ACS OMEGA
Volume 7, Issue 24, Pages 20968-20974

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsomega.2c01712

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Funding

  1. U.S. Department of Homeland Security [20CWDARI0003]

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In this work, a novel method is reported to synthesize ytterbium-doped cesium lead chloride powders, which exhibit a high X-ray scintillation light yield at room temperature. With a simple and inexpensive manufacturing process, this material shows great potential for replacing current commercial scintillators.
Ytterbium-doped cesium lead halides arc quantum cutting materials with exceptionally high photoluminescence quantum yields, making them promising materials as scintillators. In this work, we report ytterbium-doped cesium lead chloride (Yb3+:CsPbCl3) with an X-ray scintillation light yield of 102,000 photons/MeV at room temperature, which is brighter than the current state-of-the-art commercial scintillators. The high light yield was achieved based on a novel method of synthesizing Yb3+:CsPbCl3 powders using water and low-temperature processing. The combination of high light yield and the simple and inexpensive manufacturing method reported in this work demonstrates the great potential of Yb3+:CsPbCl3 for scintillation applications.

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