4.7 Article

Formation of an Electron-Phonon Bifluid in Bulk Antimony

Journal

PHYSICAL REVIEW X
Volume 12, Issue 3, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevX.12.031023

Keywords

-

Funding

  1. Agence Nationale de la Recherche [ANR-18-CE92-0020-01, ANR-19-CE30-0014-04]
  2. Jeunes Equipes de l'Institut de Physique du College de France
  3. Ile de France regional council
  4. DFG (German Research Foundation) [LO 818/6-1]
  5. Grand Eqpuipment National De Calcul IntensifCentre Informatique National de l'Enseignement Superieur (GENCI-CINES) [2020-A0090911099]
  6. Swiss National Superconducting Center [s820]

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This study discovers a two-component fluid of electrons and phonons in antimony (Sb) crystals, and highlights the dominant role of frequent momentum-conserving collisions between electrons and phonons in the transport properties.
The flow of charge and entropy in solids usually depends on collisions decaying quasiparticle momentum. Hydrodynamic corrections can emerge, however, if most collisions among quasiparticles conserve momentum and the mean-free path approaches the sample dimensions. Here, through a study of electrical and thermal transport in antimony (Sb) crystals of various sizes, we document the emergence of a two-component fluid of electrons and phonons. Lattice thermal conductivity is dominated by electron scattering down to 0.1 K and displays prominent quantum oscillations. The Dingle mobility does not vary despite an order-of-magnitude change in transport mobility. The Bloch-Gr??neisen behavior of electrical resistivity is suddenly aborted below 15 K and replaced by a quadratic temperature dependence. At the Kelvin temperature range, the phonon scattering time and the electron-electron scattering time display a similar amplitude and temperature dependence. Taken together, the results draw a consistent picture of a bifluid where frequent momentum-conserving collisions between electrons and phonons dominate the transport properties.

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