Journal
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES
Volume 142, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.physe.2022.115197
Keywords
Carbon quantum dots; Ultra-narrow bandwidth; Quantum yield; Bio-imaging
Funding
- National Natural Science Foundation of China [62164006, 11364045, 11564023, 11664044, 51904137]
- Yunnan Fundamental Research Projects [202101AS070036]
- Department of Science and Technology of Yunnan Province [2016FC001, 2019FD044]
- Yunnan local university Joint special funds for basic research [2017FH001-007, 2018FH001-017]
- Scientific Research Fund of Yunnan Education Department [2019J0563, 2019J0564, 2020Y0464, 2021Y704, 2021Y713]
- Yunnan University [2016MS14]
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Red fluorescent carbon quantum dots (R-CQDs) with ultranarrow bandwidth emission were synthesized using a one-step solvothermal method. The R-CQDs were characterized using various spectroscopic methods including photoluminescence. The photoluminescence properties of R-CQDs were found to be independent of the excitation wavelength, with the strongest emission peak at 674 nm, a full width at half maximum (FWHM) of only 23.2 nm, and a quantum yield (QY) of 7.54%. Additionally, the R-CQDs showed potential as a diagnostic marker, as they were able to enter aloe tissue. The narrow emission width and excellent QY of the R-CQDs can be attributed to the surface and edge C = O, C = N groups, as well as Ti doping. Therefore, R-CQDs have wide applications in display devices, cell labeling, and bio-imaging.
One-step solvothermal method was used to synthesize red fluorescent carbon quantum dots (R-CQDs) with ultranarrow bandwidth emission by using the titanyl-phthalocyanine (TiOPc) as the reaction precursor and ethanol as the organic solvent. We characterized the structural and optical properties of the R-CQDs by a variety of spectroscopic methods such as photoluminescence. Our studies have shown that the photoluminescence properties of R-CQDs are independent of the excitation wavelength. The strongest emission peak is at 674 nm, the full width at half maximum (FWHM) is only 23.2 nm, and the quantum yield (QY) is 7.54%. In addition, we also studied the application of the R-CQDs as a potential diagnostic marker. It was observed that the R-CQDs could enter the aloe tissue. The R- CQDs reported here have a narrow width and excellent QY characteristics, which can be attributed to the surface and edge C = O, C = N groups and Ti doping in the R-CQDs. Such R-CQDs can be widely used in the fields of display device, cell labelling and bio-imaging.
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