Journal
NATURE PHYSICS
Volume 18, Issue 6, Pages 669-+Publisher
NATURE PORTFOLIO
DOI: 10.1038/s41567-022-01628-6
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Funding
- Japan Society of the Promotion of Science (JSPS) [JP20H05619, JP18H03675]
- JSPS [JP19F19021]
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Research reveals that the low-temperature physical properties of disordered amorphous solids differ significantly from those of ordered crystalline solids. The study identifies the microscopic origin of the excess vibrational density of states, known as the 'boson peak', as quasi-localized vibrations of string-like dynamical defects.
It is widely known that the low-temperature physical properties, such as the heat capacity and thermal conductivity, of a disordered amorphous solid are markedly different from those of its ordered crystalline counterpart. However, the origin of this discrepancy is not known. One of the universal features of disordered solids is the excess vibrational density of states, known as the 'boson peak'. Here we study the microscopic origin of the boson peak through numerical investigations of the dynamic structure factor of two-dimensional model glasses over a wide frequency-wavenumber range. We show that the boson peak originates from quasi-localized vibrations of string-like dynamical defects. Furthermore, we reveal that these dynamical defects provide a common structural origin for the three most fundamental dynamic modes of glassy systems: the boson peak, fast beta relaxation and slow structural relaxation. The relation between physical properties and structure in amorphous materials is poorly understood. Simulations now show that vibrations of string-like dynamical defects likely govern the low-temperature dynamics in these systems.
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