Journal
NANO LETTERS
Volume 22, Issue 16, Pages 6509-6515Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.2c01542
Keywords
coherent phonons; van der Waals nanolayers; picosecond ultrasonics; phonon modes hybridizat i o n; hybrid nanostructures; pump-probe spectroscopy
Categories
Funding
- Engineering and Physical Sciences Research Council [EP/V05323X/1, EP/V004751/1]
- European Union
- Mercur Foundation [Pe-2019-0022]
- Deutsche Forschungsgemeinschaft [SFB TRR142/project A6, TRR160/project A1]
- Volkswagen Foundation [97758]
- University of Nottingham Anne McLaren Research Fellowship
- Royal Society Research Grant [RGS \R2\212207]
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Strain engineering using coherent phonons allows for the control of physical properties in 2D-vdW crystals, with the creation of flexural phononic crystals through periodic modulation of elastic coupling in vdW layers. Using an ultrafast pump-probe technique, we have successfully generated and detected these phonons, providing exciting prospects for ultrafast manipulation of states in 2D materials for emerging quantum technologies.
Strain engineering can be used to control the physical properties of two-dimensional van der Waals (2D-vdW) crystals. Coherent phonons, which carry dynamical strain, could push strain engineering to control classical and quantum phenomena in the unexplored picosecond temporal and nanometer spatial regimes. This intriguing approach requires the use of coherent GHz and sub-THz 2D phonons. Here, we report on nanostructures that combine nanometer thick vdW layers and nanogratings. Using an ultrafast pump-probe technique, we generate and detect in-plane coherent phonons with frequency up to 40 GHz and hybrid flexural phonons with frequency up to 10 GHz. The latter arises from the periodic modulation of the elastic coupling of the vdW layer at the grooves and ridges of the nanograting. This creates a new type of a tailorable 2D periodic phononic nanoobject, a flexural phononic crystal, offering exciting prospects for the ultrafast manipulation of states in 2D materials in emerging quantum technologies.
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