Journal
JOURNAL OF HAZARDOUS MATERIALS
Volume 432, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.jhazmat.2022.128684
Keywords
Metal-organic frameworks; Aerogel; Composites; Environmental remediation
Categories
Funding
- National Natural Science Foundation of China [51878258, 51521006]
- National Youth Foundation of China [52000064]
- Changsha Municipal Natural Science Foundation [kq2014054]
- Special Funding for the Construction of Hunan's Innovative Province [2021SK2040]
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The combination of MOFs with aerogels shows promise for environmental remediation, optimizing performance and enhancing practicality.
Environmental pollution has drawn forth advanced materials and progressive techniques concentrating on sustainable development. Metal-organic frameworks (MOFs) have aroused vast interest resulting from their excellent property in structure and function. Conversely, powdery MOFs in highly crystalline follow with fragility, poor processability and recoverability. Aerogels distinguished by the unique three-dimensional (3D) interconnected pore structures with high porosity and accessible surface area are promising carriers for MOFs. Given these, combining MOFs with aerogels at molecule level to obtain advanced composites is excepted to further enhance their performance with higher practicability. Herein, we focus on the latest studies on the MOFs@aerogel composites. The construction of MOFs@aerogel with different synthetic routes and drying methods are discussed. To explore the connection between structure and performance, pore structure engineering and quantitation of MOFs content are outlined. Furthermore, various types of MOFs@aerogel composites and their carbonized derivatives are reviewed, as well as the applications of MOFs@aerogel for environmental remediation referring to water purification and air clearing. More importantly, outlooks towards these emerging advanced composites have been presented from the perspective of practical application and future development.
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