Journal
INTERNATIONAL JOURNAL OF APPLIED CERAMIC TECHNOLOGY
Volume -, Issue -, Pages -Publisher
WILEY
DOI: 10.1111/ijac.14134
Keywords
atomic-resolution ADF STEM; depth sectioning; HPHT; III-nitride; luminescent dopant
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Funding
- KAKENHI JSPS [17H06094, 18H01823, 19H05788, 20K21073]
- Advanced Research Infrastructure for Materials and Nanotechnology in Japan (ARIM) by MEXT, Japan [JPMXP1222UT0295]
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This review discusses the point defect structures and their dynamics in wide bandgap III-nitrides, as well as the recent progress in electron microscopy.
Wide bandgap III-nitrides, such as cubic boron nitride and wurtzite-type aluminum nitride, are promising systems for optoelectronics. To extend their luminescent properties, we doped single Ce atoms into III-nitride single crystals using reactive flux with a temperature gradient method at high-pressure and high-temperature conditions. To fully understand such properties in a large size-mismatch system, it is critically important to determine the point-defect structures of single dopants, their spatial distribution in three dimensions, and their atomistic dynamics at an atomic level. This review discusses point defect structures and their dynamics in III-nitrides using single-atom-sensitive scanning transmission electron microscopy, and the recent progress in the related field of electron microscopy.
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