4.7 Article

Turbulence-induced bias in time-averaged laser absorption tomography of correlated concentration and temperature fields with a first-order correction

Journal

COMBUSTION AND FLAME
Volume 242, Issue -, Pages -

Publisher

ELSEVIER SCIENCE INC
DOI: 10.1016/j.combustflame.2022.112210

Keywords

Turbulent combustion; Absorption spectroscopy; Large-eddy simulations; Fuel chemistry

Funding

  1. Air Force Office of Scientific Research (AFOSR) Young Investigator Program [FA9550-19-1-0062, FA9550-21-1-0077]
  2. Office of Science of the U.S. Department of Energy [BES-ERCAP0021046, DE-AC02-05CH11231]

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This study examined the influence of correlated scalar fluctuations on laser absorption tomography measurements of temperature and species in a turbulent flame. It showed that bias in the measurements is primarily determined by temperature dependence in absorptivity and non-zero correlation between temperature and species concentration scalars. A first-order correction method was proposed to address these biases.
The influence of correlated scalar fluctuations on time-averaged laser absorption tomography measurements of temperature and species in a piloted turbulent premixed flame was examined using a coupled spectroscopic and fluid-dynamic analysis. To understand bias associated with turbulence, spatiotemporally resolved temperature and species mole fraction profiles predicted by large eddy simulations (LES) were used to synthetically generate time-resolved line-of-sight absorption measurements at short time scales (microsecond) to reflect the unsteady nature of a canonical jet burner across various transverse measurement planes. Inversion methods were employed on the time-averaged line-of-sight data to produce radially-resolved temperature and mole fraction profiles, analogous to those produced by laser absorption tomography performed on a time-averaged axisymmetric flowfield. It is shown that bias in the measurements compared to true time-averaged scalar fields is a function primarily of temperature dependence in absorptivity and non-zero correlation between temperature and species concentration scalars. A first-order correction to tomography measurements is proposed to account for the bias based on estimated correlations and the known spectroscopic parameters of the probed absorption transitions.(c) 2022 The Combustion Institute. Published by Elsevier Inc. All rights reserved.

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