Journal
CHEMICAL ENGINEERING JOURNAL
Volume 439, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2022.135646
Keywords
Dynamic underwater adhesive; Time-dependent performance; Self-retrieval property; Marangoni effect; Reusability
Categories
Funding
- National Science and Technology Major Project of the Ministry of Science and Technology of China [2016ZX05016]
- National Science and Technology Major Proj-ect of the Ministry of Science and Technology of China [2016ZX05046]
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We report a simple yet versatile method to fabricate underwater adhesive with time-dependent dynamic adhesion derived from silane-based polymerized deep eutectic solvent (PDES). The adhesive exhibits dynamic adhesion in underwater environments and can be tuned for optimal performance. The introduction of MXene enables near-infrared (NIR)-controlled retrieval property. This alternative strategy opens up new possibilities for designing high-performance underwater adhesive materials.
Adhesives that exhibited dynamic adhesion in underwater environments are of great importance. Here, we report a simple yet versatile method to fabricate underwater adhesive with time-dependent dynamic adhesion derived from the silane-based polymerized deep eutectic solvent (PDES). Particularly, the incorporation of silane can endow the underwater adhesive with a time-dependent adhesive performance, i.e., the adhesion strength increased at first and then decreased. With the further introduction of MXene, NIR-controlled retrieval property can be achieved. We anticipate that the alternative strategy presented here will open a new avenue for designing high-performance underwater adhesive materials with tunable and synergistic properties.
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