Journal
APPLIED PHYSICS LETTERS
Volume 121, Issue 4, Pages -Publisher
AIP Publishing
DOI: 10.1063/5.0096341
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Funding
- Shandong University [89963031]
- National Natural Science Foundation of China [52076123]
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Alloying Ga2O3 with Al2O3 to form (AlxGa1-x)(2)O-3 alloys results in diverse structural phases with distinctive optoelectronic properties. This study focuses on ordered beta-(AlxGa1-x)(2)O-3 alloys and predicts the carrier mobility and intrinsic electron mobility limit based on first principles calculations. The results show that the electron mobility of the alloys is limited by strong polar optical phonon scattering. The study provides insights into the carrier dynamics of ordered beta-(AlxGa1-x)(2)O-3 alloys and aims to improve the electron mobility for potential applications in high-power electronics.
Alloying Ga2O3 with Al2O3 yields diverse structural phases with distinctive optoelectronic properties, making them promising candidates for ultrawide bandgap semiconductors in next-generation power electronics. Yet, there is a lack of sound knowledge of the carrier dynamics in the (AlxGa1-x)(2)O-3 alloys due to their structural complexity. Herein, we focus on the ordered beta-(AlxGa1-x)(2)O-3 alloys, predict their carrier mobility, and determine the intrinsic electron mobility limit based on solving linearized Boltzmann transport equations from first principles. The predicted electron mobility for ordered beta-(Al0.25Ga0.75)(2)O-3 and beta-(Al0.5Ga0.5)(2)O-3 alloys at 300 K, respectively, is 103.6 and 80.60 cm(2)/V s, demonstrating excellent agreement with literature experiments. Such low electron mobility is limited by the intrinsically strong polar optical phonon (POP) scattering process. As the Al content further increases, the alloy's electron mobility further reduces mainly due to the enlarged Pauling ionicity, Frohlich coupling constant, and POP scattering. This work provides physical insight into the carrier dynamics in ordered beta-(AlxGa1-x)(2)O-3 alloys and seeks to improve the electron mobility for potential applications in high-power electronics. Published under an exclusive license by AIP Publishing.
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