4.8 Article

Durability Study of Thermal Transfer Printed Textile Electrodes for Wearable Electronic Applications

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 14, Issue 25, Pages 29144-29155

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.2c03807

Keywords

thermal transfer printing; laser engraving; electronic textiles; abrasion resistance; wearable RFID tag

Funding

  1. National Key R&D Program of China [2017YFE0112000]
  2. National Natural Science Foundation of China (NSFC) [51603227]

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The paper introduces a thermal transfer printing method for fabric electrodes, which overcomes the challenges of manufacturing high-performance fabric electrodes while maintaining the original characteristics of textiles. The fabric electrodes prepared by this method exhibit high conductivity, high adhesion, good abrasion/washing resistance, high patterning resolution, and good electromechanical performance.
Textile-based electronics hold great promise because they can endow wearable devices with soft and comfortable characteristics. However, the inherent porosity and fluffiness of fabrics result in high surface roughness, which presents great challenges in the manufacture of high-performance fabric electrodes. In this work, we propose a thermal transfer printing method to address the above challenges, in which electrodes or circuits of silver flake/ thermoplastic polyurethane (TPU) composites are prefabricated on a release film by coating and laser engraving and then laminated by hot-pressing to a variety of fabrics and textiles. This universal and scalable production technique enables fabric electrodes to be made without compromising the original wearability, washability, and stretchability of textiles. The prepared fabric electrodes exhibit high conductivity (5.48 x 104 S/cm), high adhesion (>= 1750 N/m), good abrasion/washing resistance, high patterning resolution (similar to 40 mu m), and good electromechanical performance up to 50% strain. To demonstrate the potential applications, we developed textilebased radio frequency identification (RFID) tags for remote identification and a large-sized heater for wearable thermotherapy. More importantly, the solvent-free thermal transfer printing technology developed in this paper enables people to DIY interesting flexible electronics on clothes with daily tools, which can promote the commercial application of smart textile-based electronics.

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