4.3 Article

A room temperature polar magnetic metal

Journal

PHYSICAL REVIEW MATERIALS
Volume 6, Issue 4, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevMaterials.6.044403

Keywords

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Funding

  1. Department of Defense, Air Force Office of Scientific Research [FA9550-18-1-0480]
  2. U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05-CH11231]
  3. Intel Corporation
  4. University of California Office of the President
  5. Ford Foundation
  6. Quantum Materials program
  7. U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231]

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The emergence of long-range magnetic order in noncentrosymmetric compounds has led to the discovery of a polar magnetic metal with unique spin textures and spin transport phenomena. The study reveals a structural transition and the emergence of a polar phase in a wurtzite-structure polar magnetic metal, which exhibits a Ned-type skyrmion lattice and a Rashba-Edelstein effect at room temperature. This discovery provides a promising new framework for investigating intriguing spin topologies and advancing spintronics.
The emergence of long-range magnetic order in noncentrosymmetric compounds has stimulated interest in the possibility of exotic spin transport phenomena and topologically protected spin textures for applications in next-generation spintronics. Polar magnets, with broken symmetries of spatial inversion and time reversal, usually host chiral spin textures. This work reports on a wurtzite-structure polar magnetic metal, identified as AA'-stacked (Fe0.5Co0.5)(5)GeTe2, which exhibits a Ned-type skyrmion lattice as well as a Rashba-Edelstein effect at room temperature. Atomic resolution imaging of the structure reveals a structural transition as a function of Co-substitution, leading to the emergence of the polar phase at 50% Co. This discovery reveals an unprecedented layered polar magnetic system for investigating intriguing spin topologies, and it ushers in a promising new framework for spintronics.

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